Materials Sciences and Applications, 2017, 8, 798-810
http://www.scirp.org/journal/msa
ISSN Online: 2153-1188
ISSN Print: 2153-117X
DOI: 10.4236/msa.2017.811058 Oct. 24, 2017 798 Materials Sciences and Applications
Electrochemical Sensors Based on Modification
of Carbon Fiber Microelectrode by Nickel
Phthalocyanine Polymer for
3-Methyl-4-Nitrophenol Analysis in Water
Yibor Fabrice Roland Bako
1
, Boukare Kabore
2
, Issa Tapsoba
1
1
Laboratoire de Chimie Analytique, Environnementale et Bio-organique (LCAEBiO), Département de Chimie,
Université Ouaga 1 Pr Joseph Ki-Zerbo, Ouagadougou, Burkina Faso
2
Bureau des Mines et de la Géologie du Burkina (BUMIGEB), Ouagadougou, Burkina Faso
Abstract
3-methyl-4-nitrophenol (MNP) is the main by-product of the organophos-
phate insecticide fenitrothion (FT), used in locust control. MNP is highly tox-
ic because it is an endocrine disruptor and then may cause adverse in the bio-
logical systems. Then, it is necessary to develop analytical methods for deter-
mination of this pollutant in the environment. In this sense, we reported
herein the development of an electrochemical sensor for the detection of
3-methyl-4-nitrophenol (MNP), one of the metabolites of fenitrothion (FT),
by using naked and modified carbon fiber microelectrode (CFME) by nickel
tetrasulfonated phthalocyanine polymer (CFME/p-NiTSPc). The voltammo-
gram showed that MNP presents one irreversible anodic peak corresponding
to the oxidation of the phenol group at 0.9 V vs Ag/AgCl. The effect of pH of
the buffer on the peak current and SWV parameters such as frequency, scan
increment and pulse amplitude were investigated in order to optimize the
electrochemical response of the sensor. The obtained results lead to the fol-
lowing optimum value: pH = 6; frequency = 25 Hz, pulse amplitude = 50 mV,
scan increment = 10 mV. With these optimum values, the calibration curves
show that the peak current varied linearly upon MNP concentration leading
to a limit of detection (LoD) for naked CFME close to 3 µg/L whereas for
CFME modified by p-NiTSPc, it reaches 0.75 µg/L. This results prove that the
presence of p-NiTSPc increasing the sensitivity of the sensor could be used to
monitor 3-methyl-4-nitro- phenol residue in real matrix.
Keywords
3-Methyl-4-Nitrophenol, Carbon Fiber Microelectrode,
How to cite this paper: Bako, Y.F.R., Ka-
bore, B. and Tapsoba I. (2017) Electrochemi-
cal Sensors Based on Modification of Carbon
Fiber Microelectrode by Nickel Phthalocya-
nine Polymer for 3-Methyl-4-Nitrophenol
Analysis in Water. Materials Sciences and
Applications, 8, 798-810.
https://doi.org/10.4236/msa.2017.811058
Received: August 24, 2017
Accepted: October 21, 2017
Published: October 24, 2017
Copyright © 2017 by authors and
Scientific Research Publishing Inc.
This work is licensed under the Creative
Commons Attribution International
License (CC BY 4.0).
http://creativecommons.org/licenses/by/4.0/
Open Access