Research Article
Synthesis, Structural Characterization, and
Preclinical Efficacy of a Novel Paclitaxel-Loaded Alginate
Nanoparticle for Breast Cancer Treatment
Ahmed A. Markeb,
1
Nagwa A. El-Maali,
1
Douaa M. Sayed,
2
Amany Osama,
3
Mohamed A. Y. Abdel-Malek,
4,5
Amen H. Zaki,
6
Mostafa E. A. Elwanis,
7
and James J. Driscoll
5,8
1
Department of Chemistry, Faculty of Science, Assiut University, Assiut 71516, Egypt
2
Department of Oncological Clinical Pathology, South Egypt Cancer Institute, Assiut University, Assiut 71516, Egypt
3
Department of Medical Biochemistry, Faculty of Medicine, Assiut University, Assiut 71515, Egypt
4
Department of Clinical Pathology, Faculty of Medicine, Assiut University, Assiut 71515, Egypt
5
Te Vontz Center for Molecular Studies, University of Cincinnati College of Medicine, Cincinnati, OH, USA
6
Department of Medical Oncology, South Egypt Cancer Institute, Assiut University, Assiut, Egypt
7
Department of Radiotherapy, South Egypt Cancer Institute, Assiut University, Assiut, Egypt
8
University of Cincinnati Cancer Institute, Cincinnati, OH, USA
Correspondence should be addressed to James J. Driscoll; driscojs@uc.edu
Received 13 January 2016; Accepted 8 August 2016
Academic Editor: Vladimir F. Semiglazov
Copyright © 2016 Ahmed A. Markeb et al. Tis is an open access article distributed under the Creative Commons Attribution
License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly
cited.
Purpose. Te antitumor activity of a novel alginate (ALG) polymer-based particle that contained paclitaxel (PTX) was evaluated
using human primary breast cancer cells. Materials and Methods. PTX was combined with ALG in a nanoparticle as a drug delivery
system designed to improve breast cancer tumor cell killing. PTX-ALG nanoparticles were frst synthesized by nanoemulsifcation
polymer cross-linking methods that improved the aqueous solubility. Structural and biophysical properties of the PTX-ALG
nanoparticles were then determined by transmission electron microscopy (TEM) and high performance liquid chromatography
(HPLC) fuorescence. Te efect on cell cycle progression and apoptosis was determined using fow cytometry. Results. PTX-
ALG nanoparticles were prepared and characterized by ultraviolet (UV)/visible (VIS), HPLC fuorescence, and TEM. PTX-
ALG nanoparticles demonstrated increased hydrophobicity and solubility over PTX alone. Synthetically engineered PTX-ALG
nanoparticles promoted cell-cycle arrest, reduced viability, and induced apoptosis in human primary patient breast cancer cells
superior to those of PTX alone. Conclusion. Taken together, our results demonstrate that PTX-ALG nanoparticles represent
an innovative, nanoscale delivery system for the administration of anticancer agents that may avoid the adverse toxicities with
enhanced antitumor efects to improve the treatment of breast cancer patients.
1. Introduction
Breast cancer is the second most common cancer worldwide,
the ffh most common cause of cancer death, and the leading
cause of cancer death in women [1]. Te global burden of
breast cancer exceeds all other cancers and the incidence
rates of breast cancer are increasing [2]. Despite signifcant
advances that have improved breast cancer detection and
treatment, women continue to die of the disease even when
disease is detected at an early stage. While locoregional
treatment has improved, there has been little progress to
improve the diagnosis and treatment of patients with sig-
nifcantly advanced disease. At present, there are limited
curative options for patients with disease that has advanced
beyond regional nodes. Novel treatment strategies, such as
nanoparticle drug delivery systems, ofer the opportunity to
enhance the delivery of anticancer therapeutics into breast
cancer cells and may eventually improve patient outcomes.
Hindawi Publishing Corporation
International Journal of Breast Cancer
Volume 2016, Article ID 7549372, 8 pages
http://dx.doi.org/10.1155/2016/7549372