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Abyssinia Journal of Science and Technology Vol. 3, No. 1, 2018, 13-19
Abyss. J. Eng. Comput. Vol. 1, No. 1, 2021, 26-30
© 2021 Kombolcha Institute of Technology, Wollo University
Characterization of Petroleum Oil Seepage Using Modern Spectroscopic
Techniques: In Case of Were Ilu-Legeheda, Ethiopia
a
*Sisay Awoke &
b
Dessalegn Gezahegn
a
Department of Chemistry, Wollo University, Ethiopia.
b
Department of Geology, Wollo University, Ethiopia.
ABSTRACT
The sedimentary regions of Ethiopia cover a significant portion of the country and comprise five distinct
sedimentary basins; namely, Ogaden, Abay, Mekele, Gambela and Southern Rift Basins. The Blue Nile
basin is a North West-South East trending branch of the Ogaden intra continental rift basin. The presence of
an oil seepage at Were Ilu and Legeheda points to the presence of an active petroleum system. The main aim
of this study was to characterize the chemical nature of the seepage oil leaked out from the hard basalt rock
of Mechela river. Seepage oil samples were analyzed using ultraviolet (UV), infrared (IR), and nuclear
magnetic resonance (NMR) spectroscopic methods. All the chemical analysis obtained from UV, IR and
NMR showed that high contents of saturated hydrocarbons were found in the petroleum collected from the
stated areas, which is the principal criterion for identification of pure petroleum oil.
Key words: Were Ilu; legeheda; petroleum; oil seepage; abay basin
INTRODUCTION
Ethiopia has five distinct sedimentary basins that
cover a significant portion of the country, namely,
Ogaden, Abay (Blue Nile), Mekele, Gambela and
Southern Rift Basins [1] [2]. The development of
most of these basins is related to the extensional
tectonic events that have taken place intermittently
since the Late Paleozoic and continued up to
Tertiary. The former three basins are presumed to
be intra continental rift basins formed as a result of
extensional stresses induced by the break-up of
Gondwana land in Upper Paleozoic [3], [4].
The Abay Basin covers an area of approximately
63,000km2 in the central northwestern plateau of
Ethiopia. It consists of Paleozoic and Mesozoic
sedimentary succession exceeding 2000 m in
thickness [5], [6]. As the basin shares the same
geotectonic origin as the Ogaden Basin, the
different strati graphic units in the Abay are nearly
similar to some of the units encountered in the
Ogaden wells [7]-[9]. Beds of marl, shale and
mudstone inter bedded with carbonates in the
lower part of the thick limestone unit (Antalo) and
upper part of the Amaba Aradom Formation (the
Upper Sandstone) are potential source rocks in the
Abay Basin [1], [2]. A geochemical analysis of an
oil seepage from Were-Ilu locality in the
northeastern margin of the basin suggests the
presence of mature oil source rock of marine
origin; possibly marine shale that has generated oil
[10]. Oil generated from the Jurassic source rocks
in the Abay Basin might be trapped by a
combination of stratigraphic and structural traps
[4], [8].
Crude oil is naturally occurring material that
comprises various hydrocarbons including
paraffins, olefins, naphthenes, aromatic and
heteroatom containing compounds as well as
organometallic compounds of nickel and vanadium
(porphyrins) [11]. Crude oil, shale oil, and sand oil
are all sources of petroleum and comprise masses
of compounds whose components can be grouped
into four essential instructions known as SARA:
Saturated hydrocarbons (alkanes and
cycloparaffins), Aromatics (with alkyl side chains),
Resins (aggregates with a large number of building
blocks which includes sulfoxides, amides,
thiophenes, pyridines, quinolines, and carbazoles),
and Asphaltenes (aggregates of prolonged
polyaromatics, naphthenic acids, sulfides,
polyhydric phenols, fatty acids, and
metalloporphyrins) [12].
However, the presence of some compounds like
polyaromatics, that are toxic or carcinogenic, sulfur
and heavy metals in high concentrations, which
have environmental implications and cause huge
Abyssinia Journal of
Engineering & Computing
*Corresponding author: sisay.awoke@wu.edu.et