CHEMICAL ENGINEERING TRANSACTIONS
VOL. 86, 2021
A publication of
The Italian Association
of Chemical Engineering
Online at www.cetjournal.it
Guest Editors: Sauro Pierucci, Jiří Jaromír Klemeš
Copyright © 2021, AIDIC Servizi S.r.l.
I SBN 978-88-95608-84-6; I SSN 2283-9216
Automotive Internal Combustion Gas Reduction using
CuZSM-5 in a Catalytic Converter
Josselyn A. Aquino Montoro
a
, Jhonny W. Valverde Flores
a,b
, Carlos A. Castañeda
Olivera
a,*
a
Escuela Profesional de Ingeniería Ambiental, Universidad César Vallejo, Av. Alfredo Mendiola 6232, Los olivos, Lima,
Perú
b
Facultad de Ciencias, Universidad Nacional Agraria La Molina, Lima, Peru
caralcaso@gmail.com
Toxic gases emitted by internal automotive combustion are responsible for air pollution and deterioration of
human health. Therefore, in this study modified zeolite was evaluated as an alternative catalyst for reducing
automotive gases in a catalytic converter. For the study, the CuZSM-5 zeolite was synthesized by the
hydrothermal method, exchanged with copper ions and then installed in the exhaust of a T3 Bi-Fuel engine.
The experiments were carried out on an auto model 1984 Toyota, with and without a catalytic converter at
different revolutions per minute (rpm) as idle, average and maximum, using the HGA 400 4GR gas analyser to
measure hydrocarbon (HC) and carbon monoxide (CO). The results showed a significant reduction in LPG
engine of Hydrocarbon Propane (78 %) and CO (60 %) at high rpm; while in gasoline engine was reduced at
Hexane (29 %) and carbon monoxide (68 %) at low rpm. This showed that Cu-zeolite is efficient in reducing
gases and more economical than the commercial converter.
1. Introduction
The expansion of cities, the industrial sector and natural factors, each year release millions of tons of air
pollutants (Pourvakhshoori, 2020). Of these, the automobile fleet is the main source of emission of toxic gases
such as carbon monoxide (CO), hydrocarbon (HC) and nitrogen oxide (NO
X
) (Bello, 2020). Multiple studies
have shown that humanity is exposed to poor air quality on a daily basis (Sánchez, 2012), inducing respiratory
and heart diseases (Valverde, 2016) and irreversible changes in the ecosystem such as loss of biodiversity
(Na, 2020).
Starting in the 19th century, catalysis was used as an alternative to mitigate and control fixed atmospheric
emissions (Zanella, 2014). Its application for mobile sources was developed with the need to eliminate diesel
engine gases through the SCR (Selective catalytic reduction) system with the injection of a reducing agent
called urea (Wang, 2015) at 32% in water, functioning as an oxidant and combustion gas reducer (Decolatti,
2012). Currently, converters are composed of precious metals such as Platinum, Rhodium and Palladium,
which behave as gas catalysts (Sen, 2016). On the other hand, these metals are highly expensive and present
rapid deactivation, which has encouraged the use of zeolite, a mineral of the three-dimensional crystalline
aluminosilicate type, with retention capacity, high selectivity and well-defined structures (Kianfar, 2020;
Moliner and Corma, 2019).
The natural zeolite proved to be efficient in the conversion of CO for gasoline engines (Rajakrishnamoorthy et
al., 2019), in reducing NOx
for diesel engines (Cho et al., 2017) and enhancement of tyre-derived oil quality
(Namchot and Jitkarnka, 2015). Likewise, the ionic exchange of zeolite with metals improves its catalytic
capacities and does not alter its morphology (Chen et al., 2018), which indicates that the metal species act as
primary active sites (Lee et al., 2019), deducing that this catalyst is more active at low temperatures, because
they present less CuO load (Pereda, 2014). As thermal support, ceramic monoliths are used, which are
usually composed of cordierite in the form of honeycombs or foams, obtained by the extrusion and corrugation
process (Govender and Friedrich, 2017). These are the most used in catalyst coating, due to their superior
hydrothermal stability, low coefficient of thermal expansion and low cost (Wang, 2015).
DOI: 10.3303/CET2186076
Paper Received: 23 September 2020; Revised: 14 March 2021; Accepted: 5 May 2021
Please cite this article as: Aquino Montoro J., Valverde Flores J.W., Castaneda Olivera C., 2021, Automotive Internal Combustion Gas
Reduction Using CuZSM-5 in a Catalytic Converter, Chemical Engineering Transactions, 86, 451-456 DOI:10.3303/CET2186076
451