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Journal of Siberian Federal University. Chemistry 3 (2019 12) 434-444
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УДК 544.472.2; 547.458.8
The Efect of Mechanical Activation and Lignin Impurities
on the Hydrolysis-Dehydration of Cellulose
in the Presence of Sibunit-4 Solid Acidic Carbon Catalysts
Nikolay V. Gromov*
а,b
,
Marina N. Denisova
c
, Tatiana B. Medvedeva
а
,
Dmitriy A. Yatsenko
a
and Oxana P. Taran
а,d,e
а
Boreskov Institute of Catalysis SB RAS,
5 Lavrentiev, Novosibirsk, 630090, Russia
b
Novosibirsk State Technical University,
20 Karl Marx, Novosibirsk, 630073, Russia
c
Institute for Problems of Chemical
and Energetic Technologies of the SB RAS
1 Sotsialisticheskaya Str., Biysk, 659322, Russia
d
Institute of Chemistry and Chemical Technology SB RAS,
FRC “Krasnoyarsk Science Center SB RAS”
50/24 Akademgorodok Str., Krasnoyarsk, 660036, Russia
e
Siberian Federal University
79 Svobodny, Krasnoyarsk, 660041, Russia
Received 31.08.2019, received in revised form 06.09.2019, accepted 10.09.2019
In the presence of acidic catalysts based on the Sibunit-4 material the efects of mechanical activation
and a lignin impurities on both the reactivity of cellulose and yields of products (monosaccharides and
furfurals) being achieved during the hydrolysis of the polysaccharide isolated by hydrotropic cooking
of miscanthus, wheat straw, and fruit shells of oats were studied. Activation was shown to signifcantly
increase the reactivity of all substrates and the yields of the target products. Impurities of lignin led to
decreasing product yields.
Keywords: hydrotropic cooking, miscanthus, oat fruit shells, wheat straw, Sibunit-4, mechanical
activation, hydrolysis, lignin, glucose, 5-hydroxymethylfurfural, xylose, furfural.
Citation: Gromov N.V., Denisova M.N., Medvedeva T.B., Yatsenko D.A., Taran O.P. The efect of mechanical activation
and lignin impurities on the hydrolysis-dehydration of cellulose in the presence of sibunit-4 solid acidic carbon catalysts,
J. Sib. Fed. Univ. Chem., 2019, 12(3), 434-444. DOI: 10.17516/1998-2836-0140.
© Siberian Federal University. All rights reserved
* Corresponding author E-mail address: gromov@catalysis.ru