IP Indian Journal of Neurosciences 2020;6(3):174–182
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IP Indian Journal of Neurosciences
Journal homepage: www.ipinnovative.com
Original Research Article
Spectroscopic and insilico Studies of Aβ (1-16) on Copper induced conformational
changes in Poly (dG-dC). Poly ( dG-dC) [Poly(GC)] DNA sequence: Implications
in Alzheimer’s disease
Govindaraju M
1,
*, Jagadeesh Kumar D
2
, Priya Narayan
2
, K R S Sambasiva Rao
3
,
K S Rao
4
1
Dept. of Molecular Biophysics Unit, Indian Institute of Science, Bengaluru, Karnataka, India
2
Dept. of Bio-Technology, Sir M. Visvesvaraya Institute of Technology, Bengaluru, Karnataka, India
3
Dept. of Biotechnology, Mizoram University (A Central University), Aizawl, Mizoram, India
4
Instituto de Investigaciones Científicas y Servicios de Alta Tecnología (INDICASAT AIP), Clayton, City of Knowledge, Panama
ARTICLE INFO
Article history:
Received 11-08-2020
Accepted 19-08-2020
Available online 18-09-2020
Keywords:
Alzheimer’s disease
DNA
Copper
Circular Dichroism
Molecular Docking
ABSTRACT
DNA molecules are dynamic and play a crucial role in life processes. DNA is polymorphic and flexible
having the ability to undergo structural changes depending on the environment. The structural property
and stability of DNA are very important for cellular functions, and are involved in normal functioning
of processes like replication, repair of DNA and protein synthesis processes. Metals like Fe and Cu are
known to play a crucial role in brain functioning and deviations in concentration from the normal are often
recognized as symptoms of malfunctions or disease. The effect of copper(Cu) and amyloid peptide (Aβ ) on
DNA in the brain has been considered very important due to their role in oxidative DNA damage, structural
changes of the Amyloid peptide and are the etiological factors for neurodegenerative diseases. In the current
investigation, changes in conformation of Poly (GC) sequence DNA induced by copper and Aβ 1-16 is
studied using Circular Dichroism (CD). CD studies have shown the shift in conformation of DNA, from B
form to an altered B-, and C-DNA conformation. The CD studies were substantiated by Molecular docking
confirms that the Aβ -copper complexes with DNA via hydrogen bond formed between Guanine-Cytosine
(GC) pairs. This work gives clues as to how copper Aβ complex modulates DNA conformations which
attributes to the stability.
© 2020 Published by Innovative Publication. This is an open access article under the CC BY-NC license
(https://creativecommons.org/licenses/by-nc/4.0/)
1. Introduction
It has been reported that in cells the predominant DNA
conformation is in its B form (Right handed), which
is known to play a pivotal role in cellular processes.
These include carrying of genetic information thereby
playing a role in Protein synthesis.
1
DNA molecule is
constantly insulted by several chemicals, metals, and
various environmental factors and studies including our
group have revealed that metals are capable of interacting
with proteins and DNA causing changes in the structure and
oxidative deterioration. Different conformations of DNA are
* Corresponding author.
E-mail address: govindaraja@iisc.ac.in (Govindaraju M).
known to exist as B, Z, C and ψ DNA. It is also known from
literature that in these different conformations, the double
helical geometry, major and minor groove depth and width
are varied.
2
The promoter regions are GC rich and over-
represented in the eukaryotic genome that forms hairpin
secondary structures, and dinucleotide repeats which are
shown to be unstable and polymorphic.
3,4
The Poly (GC)
sequence are unique class of repeats with alternating purines
and pyrimidines form secondary structures, particularly
hairpin loops that alter DNA replication and repair.
5
Under
specific conditions, the Poly (GC)) adopts a Z DNA
conformation (left handed) indicating its several roles in
cellular processes.
6–10
and lead to different neurological
disorders lead Alzheimer’s disease (AD) and Huntington
https://doi.org/10.18231/j.ijn.2020.036
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