Vol.:(0123456789)
Polymer Bulletin
https://doi.org/10.1007/s00289-019-02852-6
1 3
ORIGINAL PAPER
A new Schif’s base polymer for remediation of phenol,
2‑chlorophenol and 2,4‑dichlorophenol from contaminated
aqueous systems
Fozia K. Soomro
1
· Saima Q. Memon
1
· Najma Memon
2
· M. Y. Khuhawar
3
Received: 24 September 2018 / Revised: 1 May 2019 / Accepted: 19 June 2019
© Springer-Verlag GmbH Germany, part of Springer Nature 2019
Abstract
In the present study, a Schif’s base polymer (SBP) has been synthesized by the con-
densation of trifuoroacetylacetone and amino-polystyrene copolymer resin. After
the characterization of synthesized polymer by FT-IR spectroscopy, thermal and
elemental analyses, the removal of 2-chlorophenol (2-CP), 2,4-dichlorophenol (2,4-
DCP) along with phenol is optimized using response surface methodology. Eight-
een runs design were performed with diferent levels of variables in order to opti-
mize sorption parameters such as pH, concentration of adsorbate, agitation time and
amount of polymeric resin SBP. Maximum Langmuir sorption capacity obtained
was 110.7, 125.3 and 195.4 mg g
−1
, for phenol, 2-CP and 2,4-DCP, respectively.
Recovery of adsorbed phenol, 2-CP and 2,4-DCP was checked by diferent solvents
and was found to be quantitative (~ 99%) with methanol. The model was validated
by performing sorption experiments at optimum conditions. Kinetic and isotherm
studies of all three analytes on SBP are also discussed.
Keywords Schif’s base polymer · Sorption parameters · Polystyrene copolymer
resin · Response surface methodology · Factorial design
Introduction
In recent years, extensive use of toxic compounds produced a serious environmental
threat which demands to be solved seriously. Among these toxic compounds, phe-
nol and its chlorinated derivatives are high-priority pollutants and are registered at
* Saima Q. Memon
saimaqmemon@usindh.edu.pk
1
M. A. Kazi Institute of Chemistry, University of Sindh, Jamshoro, Pakistan
2
National Center of Excellence in Analytical Chemistry, University of Sindh, Jamshoro, Pakistan
3
Institute of Advanced Research Studies in Chemical Sciences, University of Sindh, Jamshoro,
Pakistan