Gabriel et al. Biotechnol Biofuels (2021) 14:169
https://doi.org/10.1186/s13068-021-02018-5
RESEARCH
CAZymes from the thermophilic fungus
Thermoascus aurantiacus are induced by C5
and C6 sugars
Raphael Gabriel
1,2,3
, Rebecca Mueller
1,2,3
, Lena Floerl
1,2,4,5
, Cynthia Hopson
1,2,6
, Simon Harth
1,2,7
,
Timo Schuerg
1,2
, Andre Fleissner
3,8
and Steven W. Singer
1,2*
Abstract
Background: Filamentous fungi are excellent lignocellulose degraders, which they achieve through producing
carbohydrate active enzymes (CAZymes). CAZyme production is highly orchestrated and gene expression analysis has
greatly expanded understanding of this important biotechnological process. The thermophilic fungus Thermoascus
aurantiacus secretes highly active thermostable enzymes that enable saccharifcations at higher temperatures; how-
ever, the genome-wide measurements of gene expression in response to CAZyme induction are not understood.
Results: A fed-batch system with plant biomass-derived sugars D-xylose, L-arabinose and cellobiose established
that these sugars induce CAZyme expression in T. aurantiacus. The C5 sugars induced both cellulases and hemicellu-
lases, while cellobiose specifcally induced cellulases. A minimal medium formulation was developed to enable gene
expression studies of T. aurantiacus with these inducers. It was found that d-xylose and L-arabinose strongly induced a
wide variety of CAZymes, auxiliary activity (AA) enzymes and carbohydrate esterases (CEs), while cellobiose facilitated
lower expression of mostly cellulase genes. Furthermore, putative orthologues of diferent unfolded protein response
genes were up-regulated during the C5 sugar feeding together with genes in the C5 sugar assimilation pathways.
Conclusion: This work has identifed two additional CAZyme inducers for T. aurantiacus, L-arabinose and cellobiose,
along with D-xylose. A combination of biochemical assays and RNA-seq measurements established that C5 sugars
induce a suite of cellulases and hemicellulases, providing paths to produce broad spectrum thermotolerant enzy-
matic mixtures.
Keywords: CAZy, Filamentous fungi, Thermoascus aurantiacus, Transcriptomics, Cellulase gene expression
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Introduction
Carbohydrate active enzymes (CAZymes) are vital for
the conversion of plant polysaccharides to biofuels and
bio-based chemicals [1]. Cellulose and hemicellulose are
the most abundant polysaccharides in plant biomass and
thus are an immense untapped carbon pool for biotech-
nological applications. Trough using CAZymes such as
cellulases and xylanases, lignocellulosic plant biomass
can be deconstructed into simple sugars that can be fur-
ther converted into biofuels and bioproducts [2].
Te thermophilic fungus Termoascus aurantiacus
is a notable host for thermostable CAZyme production
[3]. Te enzymes of this fungus were found to be more
heat stable and efective at deconstructing lignocellu-
lose than enzymes from other thermophilic fungi and
demonstrated the release of sugars from pre-treated bio-
mass at comparable levels to the commercial enzymatic
mixture CTec2 at 50 °C. Notably, the enzymatic mixture
from T. aurantiacus lost only half of its activity during
Open Access
Biotechnology for Biofuels
*Correspondence: swsinger@lbl.gov
1
Biological Systems and Engineering Division, Lawrence Berkeley
National Laboratory, Berkeley, CA 9720, USA
Full list of author information is available at the end of the article