VOL. 9, NO. 4, APRIL 2014 ISSN 1819-6608
ARPN Journal of Engineering and Applied Sciences
© 2006-2014 Asian Research Publishing Network (ARPN). All rights reserved.
www.arpnjournals.com
586
SYNTHESIS OF SILVER NANOPARTICLES
Raid Salih Jawaad, Khalid F. Sultan and Ali H. Al- Hamadani
University of Technology, Baghdad, Iraq
E-Mail: dr99990@yahoo.in
ABSTRACT
Widely Silver nanoparticles have been investigated because they exhibit unusual optical, electronic, and chemical
properties, depending on their size and shape, thus opening many possibilities with respect to technological applications.
The silver nanoparticle is one of the inorganic nano materials which is a good antimicrobial agents. The researcher found
that the bactericidal nano materials have opened a new epoch in pharmaceutical industries. Silver nanoparticles are the
metal of choice as they hold the promise to kill microbe’s effectively and effect on both extracellularly as well
intracellularly, the researchers by using different methods, manufactured silver nanoparticles with spherical, octahedral,
tetrahedral, hexagonal, cubic, wire, coaxial cable, triangular prism, disc, triangular mark, belt, and shell shapes.
Keywords: silver nanoparticles, surface plasmon, chemicals reduction.
1. INTRODUCTION
There are different methods to synthesize silver
nanoparticles, such as conventional temperature assisted
process, controlled reaction at elevated temperatures, and
microwave assisted process K. J. Sreeram et al., [1]
Chemical, physical synthesis methods and Bioinspired
synthesis. Chemical and physical methods lead to the
presence of some toxic chemical species adsorbed on the
surface that may have adverse effects in medical
applications. Bioinspired synthesis of nanoparticles
provides advancement over chemical and physical
methods. Microbes generally have a harder time
developing resistance to silver than they do to
antibiotics.v.Parashar et al., [2] metallic nanoparticles
shows unique properties such as excellent conductivity,
chemical stability, and catalytic activity, etc. which are
dependent on the particle size, size distribution and shape.
Among all metals, silver has the highest electrical and
thermal conductivity S. L-C Hsu, and R-T Wu [3]. The
intrinsic properties of metal nanoparticles are mainly
determined by their size, shape, composition, crystallinity,
and structure. In principle, any one of these parameters
could be controlled to fine-tune the properties of metal
nanoparticles. D. Kim et al., [4].
Green synthesis of silver NPs using , Parthenium
leaf Vyom Parashar et al., [2], citrus limon, latex of
Jatropha curcas, starch, banana peel extract, leaf extract
of Rosa rugosa, seed extract of Jatropha curcas, sucrose
and maltose, Hibiscus rosa sinensis, cochlospermum
gossypium honey and D. carotas, have been reported M.
Umadevi [5].
2. METHODS FOR PRODUCE NANO SILVER
V. Parashar. et al., [2] used fresh leaves of
Parthenium hysterophorus L. weighing 25 g were
thoroughly washed thrice in distilled water for 15 min,
dried, cut into fine pieces and were boiled in a 500 ml
Erlenmeyer flask with 100 ml of sterile distilled water up
to 5 min and were filtered, Silver nitrate (AgNO
3
) 50 ml of
fresh leaf extract was added into the aqueous solution of 1
mM Silver nitrate. Average size of the particles
synthesized was 50 nm with size range 30 to 80 nm with
irregular shape. Due to our interest to get much smaller
particles, above solution was centrifuged at a rate of 1200
rpm up to 15 minutes and investigated that particles
present in the supernatant were nearly homogenous with
average size of 7 nm silver ion complex (1mM) and leaf
extract it was observed that precursors in the ratio of 1:1
gave best results.
S. L-C Hsu, and R - T Wu [3], dissolved
AgNO
3
in de - ionized water in a beaker to this solution, a
protecting agent [poly (N - vinyl - 2 - pyrrolidone or
thiosalicylic acid or triethylamine] was added. After being
stirred, HCHO solution was then added to the solution.
Subsequently, a promoter (triethylamine or pyridine) was
added drop wise. The color of the solution turned from
clear to black. After being stirred for 200 min at room
temperature, the precipitates were washed several times
with ethanol, followed by centrifugation (6000 rpm, 10
min), to remove unbounded TEA. The particles were then
dried at room temperature under vacuum for 24 h. The
silver nanoparticles suspensions were prepared from the
dried silver nanoparticles by re-dispersing them into
alphaterpineol to prepare the nanoparticles in order to
reduce the sintering temperature. As shown in Figure-2(a),
when we used triethylamine as the reaction promoter and
TSA as the protecting agent, the silver nanoparticles were
successfully reduced from the AgNO
3
precursor. During
the preparation of Ag nanoparticle suspensions, the
individual particles had a tendency to form large
agglomerates through the van der Waals force or
Coulomb’s force. In order to prevent the agglomeration of
small particles, we added TEA to the suspensions as the
stabilizer. For TEA - protected silver nanoparticles, the
agglomeration of small particles increased with the
increasing TEA concentrations. Because the reduction
reaction of AgNO
3
by formaldehyde is slow without the
addition of basic catalysts. A higher pH is favored for
higher reducing power. In order to avoid the use of
inorganic bases as the reaction promoter, which usually
contains other unwanted metal ions, we chose organic
bases, triethylamine or pyridine as the reaction promoter.
These bases are easy to be washed out after reaction and
will not contaminate the resulting silver nanoparticles.