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Optical Materials
journal homepage: www.elsevier.com/locate/optmat
Green emission band induced by crystal defects in halogenated (-Br, -Cl, -F)
chiral imines with a benzo[b]thiophene-based moiety
B. Anzaldo Olivares
a
, O. Portillo Moreno
a,*
, G. Hernández Téllez
a
, E. Rubio Rosas
b
,
F.J. Meléndez Bustamante
c
, M.E. Castro Sánchez
c
, P. Sharma
d
, A. Mendoza
a
,
R. Gutiérrez Pérez
a,**
a
Lab. Síntesis de Complejos. Fac. Cs. Químicas., Universidad Autónoma de Puebla, Edif. FCQ-6, C.U. Av. San Claudio y 22 Sur, Col. San Manuel, C.P. 72592, Puebla, Pue,
Mexico
b
Centro Universitario de Vinculación, Universidad Autónoma de Puebla, C.P. 72570, Puebla, Pue, 72001, Mexico
c
Lab. Química Teórica, Dpto. Fisicoquímica, Fac. Cs. Quím., Universidad Autónoma de Puebla, Edif. FCQ-10, Av. San Claudio y 22 Sur, Col. San Manuel, C.P. 72570,
Puebla, Pue, Mexico
d
Instituto de Química-UNAM, Cd. Universitaria, C.P. 04510, Cd. México, Mexico
ARTICLE INFO
Keywords:
Photoluminescence
Chiral imines
Halogen efect
Crystal growth
Band gap
ABSTRACT
Four diferent chiral imines were analyzed in solid state, by changing systematically the halogen atom –X (-F, -Cl
and -Br) in the para-position of the benzene ring in the chiral moiety of benzo[b]thiophene-based imine com-
pounds. The molecular packings showed a signifcant distortion induced by the efect of the stereogenic carbon
atoms and the corresponding halogen atom, resulting in nonplanar angular-shaped small molecules.
Morphological studies by Scanning Electron Microscopy (SEM) were performed and changes in aspect and shape
of the crystals can be clearly seen. The absorbance was registered in the UV-region (~200–400 nm), and showed
typical transitions that are commonly displayed in organic molecules with π→π
*
and n→π* electronic transi-
tions. The band gap was quantifed by the Tauc model, and four electronic transitions were found, associated
with those observed in experimental results by absorbance, located in the ~3.34–5.86 eV range. By X-ray dif-
fraction (XRD) studies, a monoclinic→orthorhombic variation in the crystals was observed. Photoluminescence
(PL) signals were examined in the Vis-region at room temperature and a green emission (GE) band located in the
~450–750 nm range was observed, which was associated with crystalline defects and the existing chromo-
phores. Likewise, a PL signal located in the ~526–583 nm (~2.35–2.12 eV) range showing the shift of the green-
yellow emission was noted. By using Raman spectroscopy, the vibrational modes displayed in these crystals were
analyzed. A theoretical support of HOMO-LUMO analysis for these organic crystals is also reported.
1. Introduction
In the last three decades, a lot of research has been carried out into
organic molecules (OM) regarding their morphological, structural and
optical properties for potential application as base materials in the
construction of optoelectronic devices and organic lasers [1]. In parti-
cular, OM with emission colors in the Vis-region varying from blue [2]
and green to red have received a great deal of attention for their uti-
lization in light emitting diodes [3,4], as well as a wide range of ap-
plications [5]. However, detailed and deep analysis are always needed
and by computational theoretical calculations applying diferent
models it is possible to perform a detailed examination and predict
physical-chemical properties in these OM [6]. Most OM present dif-
ferent molecular structures generating diferent molecular packings
with the concomitant changes of the crystalline surface morphology as
well as the diferent efects generated by electrostatic interactions of
short, medium and short range [8] among other important physical
properties [7], and as such, all these facts by which absorbance and
obviously the emission optical signals can display variations. The
aforementioned properties are generally associated with molecular
structures generating signifcant changes in refectivity, refractive
index, dielectric constant, etc. [9]. Some OM in solid state are known to
have high Photoluminescence (PL) signals in the Vis-region, in parti-
cular the green emission (GE) band associated with optical and
https://doi.org/10.1016/j.optmat.2019.06.007
Received 15 January 2019; Received in revised form 8 April 2019; Accepted 6 June 2019
*
Corresponding author.
**
Corresponding author.
E-mail addresses: osporti@yahoo.com.mx (O.P. Moreno), jrgutie@correo.buap.mx (R.G. Pérez).
Optical Materials 94 (2019) 337–347
0925-3467/ © 2019 Elsevier B.V. All rights reserved.
T