Water and Environment Journal. Print ISSN 1747-6585
Water and Environment Journal 0 (2019) 1–12 © 2019 CIWEM. 1
Introduction
Today, an increasing tendency is seen in the consumption
of drugs especially antibiotics such that the drug produc-
tion has reached hundreds of thousands per year (Sun
et al. , 2009). As a result of the high rate of drug con-
sumption, its residue can enter the environment and lead
to problems. The main sources of antibiotic contamination
are the discharge of hospital, domestic, pharmaceutical,
industrial and animal wastewaters to the environment
(Ajoudanian and Nezamzadeh-Ejhieh, 2015; Arabpour and
Nezamzadeh-Ejhieh, 2015; Carabin et al. , 2015). The pres-
ence of antibiotics in water has caused drug resistance,
changes in the structure of aquatic species and interfer-
ence with the photosynthesis of plants (Aristilde et al. ,
2010; Bottoni et al. , 2010; Dirany et al. , 2010).
There are many ways to remove antibiotics from water
such as coagulation and precipitation, adsorption, nano-
filtration membrane, and biological degradation (Sun et
al. , 2009; Zazouli et al. , 2009; Arabpour and Nezamzadeh-
Ejhieh, 2015). In adsorption, pollutants are transferred
from a liquid to a solid phase without any degradation
(Chong et al. , 2010). Biological treatment requires longer
times resulting in lower yield (Belghadr et al. , 2015; Lofrano
et al. , 2017). Reverse osmosis needs high technology and
costs (Afonso-Olivares et al. , 2016). The photocatalytic
process is an advanced oxidation method that is capable
of removing various poisonous and refractory compounds
from water. In photocatalytic treatment, organic pollut-
ants are degraded in the presence of metal oxide semi-
conductors under UV and sunlight irradiation. The
photocatalytic process has the advantages such as the
ability to remove pollutants at low concentration, no need
to other chemical additives, use of sunlight and produc-
tion of no harmful materials (Chong et al. , 2010; Choi et
al. , 2014; Ye et al. , 2018).
Ciprofloxacin is one of the most widely used antibiotics
for the treatment of bacterial infections in hospitals
(Vasconcelos et al. , 2009). Ciprofloxacin cannot be
degraded biologically but it can be partially adsorbed by
biosolids in sewers, and the remainder of it can cause
health and environmental problems (Guo et al. , 2013).
Recently, many studies have been directed to develop
photocatalysts with higher yields and easier operation.
Nezamzadeh-Ejhieh and Shirazi (2014) investigated nano-
clinoptilotile particles with FeO for photocatalyst degrada-
tion for tetracycline under UV light irradiation. The
recyclable and stable CdS/C@Fe
3
O
4
photocatalyst was
synthesized by Lu et al. (2015) and was used for the
photodegradation of ciprofloxacin in water. Vaiano et al.
(2015) achieved high values of TOC removal by applying
N-doped TiO
2
doped for the treatment of spiramycin
wastewater. Yuan et al. (2016) examined TiO
2
doped with
Photodegradation of ciprofloxacin in water using photocatalyst
of zinc oxide nanowires doped with copper and cerium oxides
Maryam Mirzai, Faranak Akhlaghian & Farhad Rahmani
Department of Chemical Engineering, Faculty of Engineering, University of Kurdistan, Sanandaj, Iran
Keywords
cerium oxide; ciprofloxacin wastewater;
copper oxide; foil photocatalyst; zinc oxide
nanowires.
Correspondence
Faranak Akhlaghian, Department of Chemical
Engineering, Faculty of Engineering, University
of Kurdistan, Sanandaj 66177-15175, Iran.
Email: akhlaghianfk@gmail.com
doi:10.1111/wej.12477
Abstract
Antibiotic pollution via wastewaters has led to many environmental problems. In
this work, to remove ciprofloxacin which is an antibiotic from water, foil photo-
catalyst of zinc oxide nanowires doped with copper and cerium oxides was ap-
plied under UV light irradiation. An empirical model was developed to determine
the photocatalyst activity using response surface methodology. The independent
variables were the concentrations of precursors, copper and cerium nitrates in
the coating solution. The F-value and p-value of the model showed the accuracy
of the model. The statistical analysis indicated that copper oxide had larger ef-
fect on the response than cerium oxide. The optimized catalyst was determined
and characterized using ICP, XRD, SEM and MIP techniques. The results of this
work which are comparable to those of the previous studies have the advantage
of easy separation of the photocatalyst from water without using a centrifuge.