The electrical properties of La2CuO4/ZnO heterocontacts
at different relative humidities
Enrico Traversa
Dipartimento di Scienze e Tecnologie Chimiche, Universita' di Roma "Tor Vergata",
Via della Ricerca Scientifica, 00133 Roma, Italy
Andrea Bearzotti
Istituto di Elettronica dello Stato Solido (IESS), C.N.R., Via Cineto Romano 42, 00156 Roma, Italy
Masaru Miyayama
Research Center for Advanced Science and Technology (RCAST), University of Tokyo, 4-6-1, Komaba,
Meguro-ku, Tokyo 153, Japan
Hiroaki Yanagida
Department of Industrial Chemistry, Faculty of Engineering, University of Tokyo, 7-3-1, Hongo,
Bunkyo-ku, Tokyo 113, Japan
(Received 19 December 1994; accepted 18 May 1995)
The humidity-sensing electrical properties of heterocontacts between p-type
La
2
Cu0
4
and n-type ZnO semiconductors, and of the single oxides, as a comparison,
were studied. The heterocontacts was prepared by mechanically pressing sintered
disks of the two oxides. The electrical characterization of the heterocontacts was
carried out using dc and ac measurements at various relative humidity (RH) values, in
order to evaluate the sensing mechanisms and the electrical properties of these p-n
junctions. Their humidity sensitivity was explained in terms of the variation of the
barrier height at the p-n junctions, due to the saturation of the original interface states
by physisorbed water, which leads to the release of trapped electrons, resulting in an
increase in the forward current. The higher the number of interface states, the higher
the RH-sensitivity of the heterocontacts. Electrochemical impedance spectroscopy
(EIS) measurements showed, at 90% RH, a distribution of capacitances with different
relaxation times, which may be caused by the electrolysis of water molecules at p-n
junction sites. For their use as humidity sensors, they showed a response of 4 orders of
magnitude in the whole RH range tested, and a fast response time. The response of the
heterocontacts was bias-dependent, tunable by externally applied electric field. They
also have stand-by capability and a self-cleaning mechanism, which allow them to be
described as intelligent materials.
I. INTRODUCTION
Commercial humidity sensors currently available are
based on organic polymer films and sintered porous
ceramics,
1
which use an ionic-type humidity-sensitive
mechanism, operable at low temperatures.
2
Ceramics
have shown advantages in terms of thermal and chemical
stability, and of mechanical strength.
3
However, each of
these materials presents problems that limit their use.
One of the problems that must be overcome for
a widespread application of chemical sensors is the
surface contamination by stably adsorbed molecules,
which leads to the degeneration of their performance.
4
For humidity sensors, the detection of humidity is
dependent on water adsorption processes. Ionic-type
porous ceramics react to humidity by decreasing their
impedance due to water adsorption (chemical and physi-
cal) and/or capillary condensation within pores.
5
This
mechanism operates at low temperatures, because water
must be liquid to physisorb on the oxide surface. Because
of this mechanism, the surface resistivity of porous
ceramics increases during prolonged contact with humid
environments because of the formation of stable surface
OH" ions.
6
This drift in sensor resistance during time
makes the ceramics unreliable, unless sensor perfor-
mance is recovered by heating the material to remove the
adsorbed molecules.
7
For applications at higher tempera-
tures, other sensing mechanisms and operating principles
have been identified for ceramic oxides.
6
Electronic-
type humidity-sensitive ceramics use resistivity changes
resulting from chemisorption of water molecules, which
donate electrons to the oxide, decreasing or increasing
its resistivity according to the type of semiconducting
material (n- or /?-type).
8
These sensors can operate at
temperatures higher than 300 °C. Solid electrolyte-type
2286 J. Mater. Res., Vol. 10, No. 9, Sep 1995 © 1995 Materials Research Society