Vol.:(0123456789)
Reaction Kinetics, Mechanisms and Catalysis
https://doi.org/10.1007/s11144-019-01571-3
1 3
Reaction kinetics of mesotrione removal catalyzed by TiO
2
in the presence of diferent electron acceptors
Marina Lazarević
1
· Daniela Šojić Merkulov
1
· Vesna Despotović
1
·
Aleksandar Djordjevic
1
· Nina Finčur
1
· Nemanja Banić
1
·
Biljana Abramović
1
Received: 16 January 2019 / Accepted: 29 March 2019
© Akadémiai Kiadó, Budapest, Hungary 2019
Abstract
Many parameters infuence the reaction kinetics of photocatalytic degradation of
organic pollutants and their efects need to be evaluated. In this work, a full facto-
rial experimental design was used to study the main parameter efects in detail and
their interactions on the kinetics of mesotrione removal using TiO
2
Hombikat (TiO
2
)
suspension under simulated sunlight. The parameters which afect the efciency of
mesotrione photocatalytic degradation such as the loading of TiO
2
, concentration of
KBrO
3
, absence/presence of fullerenol (FNP), as well as O
2
purging were investi-
gated. The photocatalytic degradation efciency of mesotrione (%) in the range from
43.3 to 96.7% and apparent rate constants (k
app
), obtained by exponential ftting, in
the range from 1.849 × 10
−2
min
−1
to 6.228 × 10
−2
min
−1
with coefcient of determi-
nation ~ 0.99 are used as responses. From the statistical analysis in the case of both
responses, the highest infuence on the system has parameter loading of TiO
2
. The
highest percentage of mesotrione removal was achieved with all parameters at high
level, while the highest value of k
app
was obtained under the same experimental con-
ditions but in the absence of fullerenol.
Keywords TiO
2
photocatalysis · Kinetics · Mesotrione · Electron acceptors ·
Fullerenol · Full factorial design
Electronic supplementary material The online version of this article (https://doi.org/10.1007/s1114
4-019-01571-3) contains supplementary material, which is available to authorized users.
* Daniela Šojić Merkulov
daniela.sojic@dh.uns.ac.rs
1
Department of Chemistry, Biochemistry and Environmental Protection, Faculty of Sciences,
University of Novi Sad, Trg Dositeja Obradovića 3, 21000 Novi Sad, Serbia