Review Article Adv. Mat. Lett. 2014, 5(11), 612-628 ADVANCED MATERIALS Letters
Adv. Mat. Lett. 2014, 5(11), 612-628 Copyright © 2014 VBRI press
www.amlett.com, www.vbripress.com/aml, DOI: 10.5185/amlett.2014.4562 Published online by the VBRI press in 2014
A review on CdSe quantum dots in sensing
Pragati Malik, Jyoti Singh, Rita Kakkar
*
Computational Chemistry Laboratory, University of Delhi, Delhi 110 007, India
*
Corresponding author. Tel: (+91) 11 27666313; E-mail: rkakkar@chemistry.du.ac.in
Received: 01 April 2014, Revised: 30 June 2014 and Accepted: 30 June 2014
ABSTRACT
The primary aim of this review is to survey the literature on the ion sensing ability of quantum dots. Sensing of both cations and
anions is important, since both play significant roles in various ecological and biological processes, which makes it important to
ensure their concentration at balanced level. Contamination by heavy metal ions and various anions poses a serious threat to
humans, aquatic organisms, and to the environment; therefore detection of these ions (in presence of other cations and anions),
which are the major cause of environmental pollution is of immense significance at the present time. Owing to their enhanced
fluorescence properties and photostability, QDs offer tremendous scope to be used for ion sensing. They offer several
advantages over traditional chemical fluorophores. This review throws light on the mechanism adopted by CdSe QDs to act as
flourophores. Owing to their enhanced photoluminescence properties, QDs offer selective and sensitive determination of
various ions, which is a function of the capping on the surface of the QD nanosensor, i.e. it is possible to tune their sensing
ability by changing the capping layer, which influences the QD's interaction with various analytes. Hence, these quantum dots
may prove promising candidates in future for sensing approximately all types of analytes. Copyright © 2014 VBRI press.
Keywords: Core/shell quantum dots; analyte detection; luminescence; fluorescence; fluorophore; metal ions sensing;
photoluminescence; quantum dots quenching; nanonanosensors.
Pragati Malik has done her B.Sc. (2007) and
M.Sc. (2009) in Physical Chemistry
(specialization) from Delhi University, India
and has completed her Ph.D. under supervision
of Prof. Rita Kakkar from University of Delhi
in 2013. Her research interests include
theoretical studies of nanomaterials,
particularly CdSe quantum dots and their
interaction with various chemical and bio-
analytes in order to develop novel chemical and
biosensors.
Jyoti Singh is currently working as an
Assistant Professor in Department of
Chemistry at Hans Raj College, University of
Delhi (India). She has been teaching Physical
Chemistry for the past three years. She has
completed her Ph.D. under Prof. Rita Kakkar
from University of Delhi, India in 2010. Her
research interest includes computational
studies of quantum dots, their properties
especially their magnetism and their
applications.
Rita Kakkar, after obtaining a PhD degree in
Physical Chemistry from the University of
Delhi, undertook research on various topics.
She has been teaching Physical Chemistry at
the University of Delhi for the past three
decades. Prior to that, she taught at Miranda
House, University of Delhi. In the field of
chemistry education, she is actively involved
in designing syllabi of various universities and
conducting teacher-training workshops, and
for popularizing the use of Molecular
Modelling in teaching chemistry. Her main research interests are in
Computational Chemistry and related fields. She heads a large research
group, which is carrying out computational and experimental studies on
catalysis by nanomaterials and by enzymes. The focus of the research on
nanomaterials is to understand the growth, morphologies and stabilities of
nanocrystalline forms of metals and metal oxides, their reactivities, and
their catalytic role in various reactions, particularly those involving
degradation of organic pollutants. Her research on nanoscale materials
also includes theoretical and experimental studies on quantum dots and
their size-dependent properties for use as semiconductor devices and
sensors. Professor Rita Kakkar has over 95 research publications in
international journals. She has successfully supervised the work of 35
PhD and 7 MPhil students. She has delivered invited several talks at
scientific conferences. She also regularly reviews manuscripts for many
international journals, including those published by the American
Chemical Society, Royal Society of Chemistry, Wiley and Elsevier.