Synthesis of 2-semicarbazonomethyl-4,5-methylenedioxyphenylacetic
acids as anticonvulsant agents
Nicola Micale
a,
*, Maria Zappalà
a
, Giuseppe Zuccalà
a
, Frank S. Menniti
b
, Guido Ferreri
c
,
Giovambattista De Sarro
c
, Silvana Grasso
a
Dipartimento Farmaco-Chimico, Università di Messina, Viale Annunziata, 98168 Messina, Italy
b
Pfizer Global Research and Development, Eastern Point Road, Groton, CT 06340, USA
c
Dipartimento di Medicina Sperimentale e Clinica, Università di Catanzaro, Via T. Campanella, 88100 Catanzaro, Italy
Received 27 September 2004; received in revised form 25 November 2004; accepted 27 November 2004
Abstract
A series of 2-semicarbazonomethyl-4,5-methylenedioxyphenylacetic acids (12–19) were synthesized and tested as anticonvulsant agents
in DBA/2 mice against sound-induced seizures and the results compared to those previously reported for the corresponding methyl esters
(4-11). The new compounds possess anticonvulsant properties lower than those of 4–11, but, in some instances, comparable to that of GYKI
52466, a well-known noncompetitive AMPA receptor antagonist.
© 2005 Elsevier SAS. All rights reserved.
Keywords: 4,5-Methylenedioxyphenylacetic acids; Anticonvulsant activity; AMPA antagonists
1. Introduction
Epilepsy, one of the most frequent neurological afflictions
in man characterized by excessive temporary neuronal dis-
charges resulting in uncontrolled convulsion, requires spe-
cial medical attention. Although several new anticonvulsants
are already in clinical use, some types of seizures are still not
adequately treated with current therapy. Toxicity, intoler-
ance, and lack of efficacy for certain types of seizure are some
of the limitations of the current medications [1].
Drugs effective against the most common forms of epilep-
tic seizures appear to work by limiting the sustained repeti-
tive firing of a neuron by one of the following mechanisms:
(i) enhancement of GABA-mediated synaptic inhibition, (ii)
stabilization of the inactivated state of voltage-operated Na
+
channels, (iii) inactivation of voltage-activated Ca
2+
chan-
nels.
Considerable interest has recently been focused on antago-
nists of the ionotropic glutamate receptors (NMDA, AMPA
and KA) having significant anticonvulsant activity thus pro-
viding the basis for an extensive research in this area.
GYKI 52466 (1, 1-(4-aminophenyl)-4-methyl-7,8-
methylenedioxy-5H-2,3-benzodiazepine) and its analogues
such as GYKI 53655 (2)(Fig. 1), acting as noncompetitive
antagonists of the AMPA receptors [2,3], displayed potent
anticonvulsant properties [4,5] and this induced growing inter-
est on 2,3-benzodiazepine derivatives.
Since some time our research group is involved in the
search of new noncompetitive AMPA receptor antagonists
containing the 2,3-benzodiazepine skeleton [6–8].
Based on the anticonvulsant properties of the previously
described [7] 1-(4-aminophenyl)-3,5-dihydro-3-N-methyl-
carbamoyl-7,8-methylenedioxy-4H-2,3-benzodiazepin-4-
one (3), we recently designed and tested [9,10] a series of
alkyl esters of 4,5-methylendioxyphenyl acetic acid (e.g.,
4–11) bearing an N-alkyl-(thio)semicarbazonomethyl moi-
ety at position 2, which may be envisaged as “open models”
of reference compound 3 (Fig. 1). Within this series of deriva-
tives, methyl ( Z)-2-[(4-aminophenyl)-(4-methylsemi-
carbazono)-methyl]-4,5-methylenedioxyphenyl-acetate 11
proved to be the most active compound. It displayed an anti-
convulsant activity slightly higher than that of its parent 3
and 5-fold higher than that shown by reference compound
GYKI 52466.
* Corresponding author.
E-mail address: nmicale@pharma.unime.it (N. Micale).
Il Farmaco 60 (2005) 231–235
http://france.elsevier.com/direct/FARMAC/
0014-827X/$ - see front matter © 2005 Elsevier SAS. All rights reserved.
doi:10.1016/j.farmac.2004.11.012