PHYSICAL REVIEW E 106, 014706 (2022)
Anisotropic viscous effects of local flow by a rotating microparticle in nematic liquid crystal
Jun-Yong Lee ,
1
Jae Hoon Lee,
1
Bohdan Lev ,
2
and Jong-Hyun Kim
1, 3 , *
1
Department of Physics, Chungnam National University, 99 Daehak-ro, Yuseong-gu, Daejeon, 34134, Korea
2
Bogolyubov Institute for Theoretical Physics of the NAS of Ukraine, Metrolohichna Str.14-b, Kyiv, 03680, Ukraine
3
Institute of Quantum Systems, Chungnam National University, Daejeon, 34134, Korea
(Received 10 October 2021; revised 16 May 2022; accepted 29 June 2022; published 25 July 2022)
The presented study opens a perspective to investigate the effects of local flow on nematic liquid crystals. A
particle rotated in nematic fluids typically generates a rotationally symmetric local flow, which causes a change
in the director orientation. The director above the threshold velocity has a particular angle determined by the ratio
of Leslie coefficients, α
2
/α
3
. In 5CB liquid crystals, this director angle with respect to the flow is approximately
13
◦
. The angle is calculated through Ericksen-Leslie theory. The angle is not dependent on rotation frequency or
particle size but temperature. The area of the influenced region increases with the rotation frequency and particle
size. The changes in radius of the influenced region are calculated theoretically using Ericksen number. Further,
an interference pattern appears at the edge of the influenced region by the refractive indexes mismatch between
the influenced region and the rest. We experimentally obtain the thickness of the influenced region analyzing
intervals of the pattern.
DOI: 10.1103/PhysRevE.106.014706
I. INTRODUCTION
Nematic liquid crystals (NLCs) have not only fluidity but
also long-range orientational ordering between molecules,
which distinguishes them from isotropic fluids. The most
remarkable features of NLCs are an appropriate degree of
elasticity and various anisotropies on the macroscopic scale
[1,2]. Liquid crystal (LC) molecules tend to align in an orien-
tation similar to that of adjacent molecules, where the average
orientation is called the director. The director can be con-
trolled by external fields, the properties of the substrates in
which the LCs are constrained, and so on [3]. Furthermore,
flow is also one of the most important factors that influence
the director; in particular, the direction and gradient of the
flow play a critical role. We can observe not only changes
in the alignment of the director but also various instabilities
of the system by generating a flow in a uniformly aligned LC
cell [4–9]. Rich responses of the LC director can result from
different types of shear flow and shapes of the cell confining
the LCs [10–15].
In nematic fluid research, the anisotropy of viscosity in
addition to flow is also important. Anisotropy of viscosity
can be expressed through Miesowicz viscosity and Leslie
coefficients, and the hydrodynamics of nematic fluids can
be analyzed through the theories from Ericksen and Leslie
[16–20]. From anisotropic viscosity, we can observe many
interesting phenomena that do not appear in isotropic fluids
[21–26]. For example, a Poiseuille flow in a uniformly and
obliquely aligned LC to the flow creates transverse pressure
[27]. Additionally, because the sign and magnitude of the
coefficients play an important role in determining the size
*
Corresponding author: jxk97@cnu.ac.kr
or orientation of the phenomena, many studies on various
physical quantities of LCs have been conducted [28–32].
To date, most research on the behavior of LCs has focused
on large-scale flow, while the effects of local flow on LCs
have received relatively less attention. Among the studies
on the effects of local flow, Rovner et al. observed various
phenomena resulting from dispersed ferromagnetic discs ro-
tated by a magnetic field in uniformly aligned LCs [33]. They
pointed out that the alignment of the director around each disc
changes when the angular velocity of the disc exceeds a cer-
tain threshold, and also that the relaxation of the phenomena
is affected by the ratio between elasticity and viscosity when
rotation is stopped [33]. However, they did not investigate
the alignment change of the director further or the cause of
the change in detail. In the present work, we experimentally
generate a local flow on the single-particle scale using micro-
sized ferromagnetic spheres in NLCs and a rotating magnetic
field. We apply Ericksen-Leslie theory on this scale and reveal
not only the details of the director alignment in the region
where the flow exceeds the threshold velocity and its cause
but also the shape of the region where the alignment change
happens. The related phenomena are calculated through the
viscous torque exerted on the director and the proposed model
that considers the distance from the substrate in the Ericksen
number.
II. EXPERIMENTS
We used a mixture of NLCs and spherical ferromagnetic
particles in a rotating magnetic field to generate a local flow.
The mixture was prepared through the following process.
Ferromagnetic spheres approximately 8–30 μm in diameter
were dispersed into deionized water at a concentration of 1%.
The ferromagnetic spherical particles (CFM-80-5 and CFM-
2470-0045/2022/106(1)/014706(9) 014706-1 ©2022 American Physical Society