Characterizaton of recombinant Bacillus halodurans CM1 xylanase
produced by Pichia pastoris KM71 and its potental applicaton in
bleaching process of bagasse pulp
Haniyya
1
, Lina Mulyawat
1
, Is Heliant
1,*
, Phitsanu Pinmanee
2
, Kanokarn Kocharin
3
, Duriya Cantasingh
2
, Thidarat Nimchua
2
1
Center for Bioindustrial Technology, Agency of Assessment and Applicaton of Technology (BPPT), Building 611/614, LAPTIAB‐BPPT,
PUSPIPTEK Area, Setu, South Tangerang 15314, Indonesia
2
Enzyme Technology Research Team, Biorefnery and Bioproduct Technology Research Group, Natonal Center for Genetc Engineering and
Biotechnology,113 Phahonyothin Road, Khlong Nueng, Khlong Luang, Pathum Thani 12120, Thailand
3
Microbial Cell Factory Research Team, Biorefnery and Bioproduct Technology Research Group, Natonal Center for Genetc Engineering
and Biotechnology, 113 Phahonyothin Road, Khlong Nueng, Khlong Luang, Pathum Thani 12120, Thailand
*Corresponding author: is.heliant@bppt.go.id
SUBMITTED 9 July 2020 REVISED 19 October 2020 ACCEPTED 10 December 2020
ABSTRACT Thermoalkalophilic xylanases promise potental applicaton in pulp biobleaching to reduce the use of toxic
chlorinated chemical agents, which are harmful to the environment. In this study, a thermoalkalophilic endoxylanase gene
(bhxyn3) originatng from Indonesian indigenous Bacillus halodurans CM1 was cloned into yeast expression vector pPICZα A
and expressed in Pichia pastoris KM71 under the control of AOX1 promoter. Recombinant P. pastoris expressed the highest
fnal level of xylanase (146 U/mL) on BMGY medium afer fve days of cultvaton. Optmizaton of xylanase producton on a
small scale was carried out by varying the methanol concentratons and the optmal xylanase producton by the recombinant
P. pastoris was observed in the culture with 2% (v/v) methanol afer four days of the inducton phase. The recombinant
xylanase (BHxyn3E) was thermotolerant and alkalophilic, with an optmal temperature at around 55‐65 °C and under pH 8.0.
The enzyme actvity was slightly induced by K
+
, Fe
2+
, and MoO
4
2‐
. Enzymatc bleaching of bagasse pulp with no prior pH
adjustment (pH 9) using BHxyn3E at 200 U/g oven dried pulp increased the lightness index (L*) and changed substantally
the color a index (a*); however, the treatments did not change the whiteness index in a signifcant way. Therefore, further
optmizaton and assessment such as adjustment of incubaton temperature and pH in biobleaching were needed to reduce
the use of harmful chemical agents in industrial applicatons.
KEYWORDS Bacillus halodurans; biobleaching; cellulase‐free xylanase; Pichia pastoris; thermoalkalophilic xylanase
Indonesian Journal of Biotechnology
VOLUME 26(1), 2021, 15‐24 | RESEARCH ARTICLE
1. Introducton
Remarkable interest has been focused on integrating hy
drolytic enzymes, such as xylanases, that degrade xylan
components in plant cell walls into noncomplex sugars
in industries, particularly in the pulp and paper industry.
Xylanases (EC 3.2.1.8) are produced by microorganisms
and considered as the key enzymes that hydrolyze β1,4
xylans to lead to the degradation of complex polysaccha
rides (Jeya et al. 2009). On the other hand, the enzymes
have widespread potential applications to be used in such a
wide range of industrial fields (textile, feed, beverage, and
biofuels) since its ability to facilitate the removal of xy
lan through partial hydrolysis of lignin carbohydrate com
plexes, thereby enabling lignin removal from raw materi
als allowing it to be processed in the next stages of man
ufacturing. In the pulp and paper process, this fragmenta
tion of xylan polymer allows residual lignin attached to the
remaining xylan complex, to be exposed by the efficient
used bleaching agents. Thus, pretreatment of pulp using
xylanases can reduce the load of chlorine and chlorine
based compounds in the subsequent chemical bleaching
stages. As a side effect, the utilization of cellulasefree xy
lanase enable to enhance several physical pulp properties,
such as brightness, tensile strength, and tear factor with
out affecting the cellulose fiber strength of paper products
(Zhao et al. 2015).
Currently, xylanases that are intended to be used in the
industrial bleaching process must be robust to operate in
extreme conditions since most operations were conducted
under high temperature and strong alkaline pH for at least
anhour long. Hence it must be adaptable in such an ex
treme environment. Xylanases are produced by members
of bacteria and fungi, commonly in group of bacterial xy
lanases display an active at mesophilic temperatures (be
low 50 °C) in acidic or neutral pH (Walia et al. 2017).
Indones J Biotechnol 26(1), 2021, 15‐24 | DOI 10.22146/ijbiotech.57701
www.jurnal.ugm.ac.id/ijbiotech
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