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ISSN 1063-7745, Crystallography Reports, 2016, Vol. 61, No. 3, pp. 414–420. © Pleiades Publishing, Inc., 2016.
Original Russian Text © L.A. Dadinova, E.V. Rodina, N.N. Vorobyeva, S.A. Kurilova, T.I. Nazarova, E.V. Shtykova, 2016, published in Kristallografiya, 2016, Vol. 61, No. 3,
pp. 406–412.
Structural Investigations of E. Coli Dihydrolipoamide Dehydrogenase
in Solution: Small-Angle X-Ray Scattering and Molecular Docking
L. A. Dadinova
a,b
, E. V. Rodina
b
, N. N. Vorobyeva
b
, S. A. Kurilova
b
, T. I. Nazarova
b
, and E. V. Shtykova
a,b
a
Shubnikov Institute of Crystallography, Russian Academy of Sciences, Leninskii pr. 59, Moscow, 119333 Russia
b
Moscow State University, Moscow, 119992 Russia
e-mail: shtykova@ns.crys.ras.ru
Received December 10, 2015
Abstract—Dihydrolipoamide dehydrogenase from Escherichia coli (LpD) is a bacterial enzyme that is
involved in the central metabolism and shared in common between the pyruvate dehydrogenase and 2-oxo-
glutarate dehydrogenase complexes. In the crystal structure, E. coli LpD is known to exist as a dimer. The
present work is focused on analyzing the solution structure of LpD by small-angle X-ray scattering, molecular
docking, and analytical ultracentrifugation. It was shown that in solution LpD exists as an equilibrium mix-
ture of a dimer and a tetramer. The presence of oligomeric forms is determined by the multifunctionality of
LpD in the cell, in particular, the required stoichiometry in the complexes.
DOI: 10.1134/S1063774516030093
INTRODUCTION
Dihydrolipoamide dehydrogenase (LpD) is a fla-
vin-containing protein that catalyzes the oxidation of
the SH group of lipoamide in oxidoreductases to form
an S–S bond. The flavin cofactor (FAD) of LpD is
reduced to FADH
2
, and its reverse conversion requires
the presence of NAD
+
. Dihydrolipoamide dehydroge-
nase is involved in three different multienzyme com-
plexes that catalyze similar decarboxylation reactions
of 2-oxoacids. All of these complexes comprise three
enzymes known as Е1, Е2, and Е3, where LpD is the
Е3 component and the E2 subunit is used by LpD as
the lipoamide-containing protein substrate. The Е1
and Е2 subunits have different structures in different
complexes, whereas the Е3 protein is essentially the
same in all of the complexes [1–4]. The two main Е3-
containing complexes play an essential metabolic role.
Thus, they link the utilization of carbohydrate sub-
strates to oxidative phosphorylation. The pyruvate
dehydrogenase complex (PDC) converts pyruvate (the
glycolysis product) to Ас-СоА (the main substrate of
the Krebs cycle). The 2-oxoglutarate dehydrogenase
complex catalyzes one of the reactions in the Krebs
cycle. The pyruvate dehydrogenase complex from
Gram-negative bacteria (for example, from E. coli) is
composed of 24 E1 subunits and 24 E2 subunits,
whereas the multiplicity of E3 remains unknown.
According to different estimates, there are 12 [5, 6] or
24 [7–9] E3 subunits; i.e., E3 may consist of six
dimers or six tetramers. Meanwhile, all of the Е3
enzymes function as dimers, and their active site con-
tains the reactive disulfide bridge, which is directly
involved in catalysis [10]. These reactions are essential
for aerobic respiration. Dihydrolipoamide dehydroge-
nase plays an equally important role in anaerobic
organisms, since this enzyme is involved in the syn-
thesis of branched-chain keto and amino acids. The
E3 enzyme was also found in the absence of multien-
zyme complexes, for example, in organisms lacking
2-oxoacid dehydrogenase [11, 12]. These properties
attest to the multifunctional character of LpD. The
crystal structure of E. coli LpD was determined at
2.5-Å resolution [10], and it was shown that LpD
exists as a dimer in the crystalline state (PDB ID:
4JDR). However, the solution structure of this protein
was unknown.
Since all vitally essential reactions of enzymes
occur in a liquid medium, the aim of the present study
is to investigate the behavior of LpD in solution, i.e.,
under near-physiological conditions, by small-angle
X-ray scattering (SAXS). The SAXS method is suit-
able for the determination of a complex molecular
architecture of proteins even in a multicomponent
solution [13]. Modern techniques for the interpreta-
tion of SAXS data provide information about the qua-
ternary structure of biological objects. For example,
molecular tectonics can be employed to determine the
structures of macromolecular complexes composed of
subunits with known or partially known atomic struc-
tures [13–16]. However, it should be taken into
account that different models may be reconstructed
from the same SAXS curve because the recovery of a
three-dimensional object from a one-dimensional
curve is obviously ambiguous [17]. In order to reduce
the ambiguity in the interpretation of the SAXS data,
STRUCTURE OF MACROMOLECULAR
COMPOUNDS