Vol.:(0123456789) 1 3
Clean Technologies and Environmental Policy
https://doi.org/10.1007/s10098-018-1523-5
ORIGINAL PAPER
Green technology of liquid biphasic fotation for enzyme recovery
utilizing recycling surfactant and sorbitol
Revathy Sankaran
1
· Pau Loke Show
1
· Yee Jiun Yap
2
· Yang Tao
3
· Tau Chuan Ling
4
· Katsuda Tomohisa
5
Received: 18 December 2017 / Accepted: 22 March 2018
© Springer-Verlag GmbH Germany, part of Springer Nature 2018
Abstract
Liquid biphasic fotation (LBF) system has been recognized as an efcient, green, economically sustainable and biocompat-
ible technique for biomolecules separation and purifcation. The main drawbacks of the conventional process of biomolecules
separation are expensive production cost, utilization of phase components that are inefciently recycled and global pollution
due to high chemical consumption and wastage. In this paper, a novel approach of LBF system for lipase recovery utilizing
recycling phase components comprising surfactant and xylitol was investigated. The scope of this study focuses on pollution
prevention as well as clean and environmentally friendly process for enzyme extraction via LBF. The green process proposed
in this study uses phase-forming components that have recovery and recycling abilities for minimal use of chemicals for
enzyme extraction. This novel method utilized Triton X-100 and xylitol for lipase extraction from Burkholderia cepacia. A
few parameters were optimized to obtain high lipase separation efciency and yield. Based on the ideal conditions of LBF,
the average lipase separation efciency and yield are 86.46 and 87.49%, correspondingly. Phase components recycling were
proposed in order to reduce the chemicals consumption in LBF system. Upscaling of the recycling study exhibited consistent
result with the laboratory scale. It was found that 97.20 and 98.67% of Triton X-100 and xylitol were recovered after fve
times of recycling and that a total of 75.87% of lipase separation efciency was obtained. Recovery and recycling of phase
components in the extraction process are established as the principal green chemistry method, which yields high separation
efciency and is economically feasible on an industrial scale.
Keywords Liquid biphasic fotation · Green · Recycling phase components · Surfactant · Xylitol
Introduction
Traditional purifcation methods such as monoliths, column
chromatography, crystallization, diafltration, membrane
separation and precipitation are generally time-consuming,
involves batch operation, requires multi-step operations and
generates low concentration of products, and the products
are often combined in complex mixtures of impurities (Nfor
et al. 2008). Due to these limitations, industries today are
looking for an alternative purifcation method that is sim-
ple and inexpensive and generates a high yield of products
with low environmental impacts (Gupta et al. 2004). Liq-
uid biphasic fotation (LBF) is comparatively an innova-
tive extraction and purifcation technique that fuses solvent
sublation (SS) with aqueous two-phase system (ATPS)
(Sankaran et al. 2018). This novel method is introduced as
an alternative to conventional liquid–liquid extraction (Bi
et al. 2009).
* Pau Loke Show
PauLoke.Show@nottingham.edu.my
1
Department of Chemical and Environmental Engineering,
Faculty of Engineering, University of Nottingham
Malaysia Campus, Jalan Broga, 43500 Semenyih,
Selangor Darul Ehsan, Malaysia
2
Department of Applied Mathematics, Faculty of Engineering,
University of Nottingham Malaysia Campus, Jalan Broga,
43500 Semenyih, Selangor Darul Ehsan, Malaysia
3
College of Food Science and Technology, Nanjing
Agricultural University, Nanjing, Jiangsu, China
4
Faculty of Science, Institute of Biological Sciences,
University of Malaya, 50603 Kuala Lumpur, Malaysia
5
Department of Chemical Science and Engineering, Kobe
University, Kobe 657-8501, Japan