1 3
Mine Water Environ
DOI 10.1007/s10230-016-0424-2
TECHNICAL ARTICLE
Characterization and Toxicity Assessment of Wastewater
from Rock Phosphate Processing in Tunisia
Ali Mekki
1
· Asma Awali
1
· Fathi Aloui
1
· Slim Loukil
1
· Sami Sayadi
1
Received: 4 July 2016 / Accepted: 14 November 2016
© Springer-Verlag Berlin Heidelberg 2016
Burnett 1994). Gnandi and Tchangbedji (2006) observed
that some diseases, such as dental luorosis in children, are
strongly related to the luoride in the phosphate rock. Also,
ine phosphate particles generated by mining have been
found to negatively afect the human respiratory system
(Pope and Burnett 2002). McDonnell et al. (2000) showed
that they contribute to the incidence of cancer, while others
have found that they can cause respiratory diseases, such as
bronchitis and asthma (Herich and Holscher 2002).
With over a century of experience in mining, upgrad-
ing, and marketing Tunisian phosphates, the Company of
Phosphates of Gafsa (CPG), is one of the world’s leading
phosphate producers (Narasiah et al. 1988). Production
exceeded 8 million metric tons (t) in 2010, making CPG
the world’s ifth largest phosphate producer (Tijani and
Fakhfakh 2011), though social unrest in Tunisia has sub-
sequently afected production. The CPG works 10 surface
mines in ive phosphate ields, all in the same Eocene geo-
logical level, principally based around deposits in the Gafsa
basin in southern Tunisia (Tijani and Fakhfakh 2011). The
phosphate is ‘washed’ in several phases, including mechan-
ical separation and treatment, to increase the P
2
O
5
content
(Narasiah et al. 1988). This consumes 5 t of water per ton
of phosphate. However, of these 5 t of water, 3.65 t were
recycled, 0.15 t accompanies the phosphates product as
moisture, and 1.2 t are lost (Narasiah et al. 1988).
Thus, production of 8 million tons per year of market-
able phosphate consumes approximately 10.5 million tons
of waters (Tijani and Fakhfakh 2011). Moreover, the water
that is being used by CPG is paleowater from Inill Conti-
nental, and is not renewable (Tijani and Fakhfakh 2011). In
this study, we characterized CPG’s wastewater from phos-
phate ore processing (WWPP) and investigated its efects
on the receiving environment, in particular the soil, in order
to develop a suitable water treatment process.
Abstract Phosphate ore processing wastewater (WWPP)
from the Gafsa phosphate region of Tunisia was charac-
terized. The WWPP had a very high turbidity, an almost
neutral or slightly alkaline pH, and high salinity. The aver-
age chemical and biochemical oxygen demands (COD and
BOD) met wastewater discharge standards, but the COD/
BOD5 (4.34) signiicantly exceeded biodegradability val-
ues. Total nitrogen, residual phosphorus, and some oth-
ers chemical constituents exceeded wastewater discharge
standards. Microbiological enumeration showed that the
eluents were very low in microlora. Untreated WWPP
and diluted (WWPP/4) inhibited bioluminescence of
Vibrio fischeri by 76 and 45%, respectively. The WWPP
had a phytotoxicity rate of 20–70%, respectively, for alfalfa
and tomato seeds. Adding the eluent to soil for 60 days
reduced the residual phytotoxicity of the WWPP-irrigated
soil to about 15 and 34%, respectively, for tomato and
alfalfa seeds.
Keywords Waste water · Phosphate industry · Salinity ·
Toxicity · Soil
Introduction
The phosphate industry is the cause of many environmen-
tal problems (Lipfert et al. 2000; Pope and Burnett 2002).
Natural phosphates contain many metallic elements, some
of which can negatively afect the environment (Jarvis and
* Ali Mekki
a_mekki_cbs@yahoo.fr
1
Laboratory of Bioprocesses, Center of Biotechnology
of Sfax, AUF (PER-LBP), BP 1177, 3018 Sfax, Tunisia