Insights into the carbonate effect on water
oxidation over metal oxide
photocatalysts/photoanodes
Hitoshi Kusama,*
a
Masanori Kodera,
a
Koichi Yamashita
b
and Kazuhiro Sayama
a
a
Global Zero Emission Research Center (GZR), National Institute of Advanced
Industrial Science and Technology (AIST), AIST Tsukuba West, 16-1 Onogawa,
Tsukuba, Ibaraki 305-8569, Japan
b
Element Strategy Initiative for Catalysts and Batteries (ESICB),
Kyoto University, Nishikyo-ku, Kyoto 615-8245, Japan
Supplementary information
Table S1 Summary of the effect of carbonate on a photocatalyst and (photo)anode
using TiO2 and BiVO4
Semiconductor TiO2 BiVO4
Photocatalytic activity for water splitting into H2 and O2 Yes No
a
Improvement of photocurrent Yes Yes
H2O2 production on photoanode Yes
b
Yes
H2O2 production on anode in the dark Yes Yes
a
BiVO4 photocatalyst cannot evolve H2 because of the positive conduction band.
b
Data in this work.
1
Electronic Supplementary Material (ESI) for Physical Chemistry Chemical Physics.
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