RESEARCH ARTICLE
Effect of cell compression on the performance of a non–hot‐
pressed MEA for PEMFC
Naveen K. Shrivastava
1
| Abheek Chatterjee
2
| Tequila A.L. Harris
3
1
Department of Mechanical Engineering,
Birla Institute of Technology and Science,
Pilani‐Dubai Campus, UAE
2
Department of Mechanical Engineering,
National Institute of Technology,
Warangal 506004, India
3
George W. Woodruff School of
Mechanical Engineering, Georgia Institute
of Technology, Atlanta, GA 30332, USA
Correspondence
Tequila A. L. Harris, George W. Woodruff
School of Mechanical Engineering,
Georgia Institute of Technology, Atlanta,
GA 30332, USA.
Email: tequila.harris@me.gatech.edu
Funding information
National Science Foundation, Grant/
Award Number: CMMI‐095339
Summary
In this study, the effect of cell compression on the performance of a non–hot‐
pressed membrane electrode assembly (MEA) for a polymer electrolyte mem-
brane fuel cell (PEMFC) is presented. The MEA is made without hot pressing,
by carefully placing the gas diffusion electrodes (GDEs) and a membrane in a
fuel cell fixture. Cell performance is assessed at five different compression
ratios between 3.6% and 47.8%. It has been shown that ohmic resistance of
the cell, mass transport resistance of reactants, charge transfer resistance at
electrode, and overall cell performance are strongly dependent on the cell com-
pression. On increasing the cell compression gradually, cell performance
improves initially, reaches the best, and then deteriorates. The cell performance
is assessed at fully humidified condition and at dry condition. Optimum cell
performances are obtained at compression ratios of 14.2% and 25.7% for 100%
relative humidity (RH) and 50% RH, respectively. It is also found that the cell
with proper compression and at fully humidified conditions can deliver similar
performance to a conventional hot‐pressed MEA. Finally, it is shown that after
the tests, GDEs can be peeled out, and the membrane inspection can be done as
a postexperimental analysis.
KEYWORDS
compression, degradation, gas diffusion electrode, gasket, polymer electrolyte membrane, polymer
electrolyte membrane fuel cell
1 | INTRODUCTION
Research on nonconventional energy sources such as fuel
cells has drastically increased in the recent past due to the
depletion of fossil fuel‐based conventional energy sources
and the pollution concerns associated with them.
1
Poly-
mer electrolyte membrane fuel cells (PEMFCs) are among
the most advanced fuel cell technologies. These are prom-
ising for both stationary and portable applications due to
various advantages, including low operating temperature,
rapid startup and shut‐down, high power density, high
efficiency, and noise and pollution free operation.
1-4
Despite the significant progress that has been made, there
still remain critical issues and challenges, such as cost,
durability, cold start capability, water and thermal man-
agement, which must be addressed in order to achieve
the widespread commercialization of the PEMFCs.
3,5
In a fuel cell, gaskets are used between membrane elec-
trode assembly (MEA) and flow field plate to avoid gas
leakage. All the cell components (membrane, gas diffusion
electrodes [GDE], flow field plates, current collectors, and
end plates along with gaskets) are held together firmly with
several nuts and bolts to make better electrical contact
between all the components. Cell assembly pressure, bolt
torque, thickness of the gasket applied between the MEA,
and flow field plates are interrelated. Mostly, carbon cloth
Received: 16 May 2019 Revised: 24 September 2019 Accepted: 25 September 2019
DOI: 10.1002/er.4933
Int J Energy Res. 2019;1–18. © 2019 John Wiley & Sons, Ltd. wileyonlinelibrary.com/journal/er 1