Journal of Geoscience and Environment Protection, 2022, 10, 121-135
https://www.scirp.org/journal/gep
ISSN Online: 2327-4344
ISSN Print: 2327-4336
DOI: 10.4236/gep.2022.109008 Sep. 27, 2022 121 Journal of Geoscience and Environment Protection
Adsorption of Chromium (VI) Using
Nano-ZnO Doped Scrap Tire-Derived
Activated Carbon
Jean Tsitsi Chigova, Stanford Mudono
Department of Chemical Engineering, Faculty of Engineering, National University of Science and Technology (NUST),
Bulawayo, Zimbabwe
Abstract
Nowadays, nano mineral modified biochars show a promising adsorption
capacity for pollutants removals by combining the advantages of porous struc-
ture of biochar and unique property of nano minerals. In this work, nano-
zinc oxide doped scrap tire derived activated carbon (nZnO-STAC) was syn-
thesized by wetness impregnation method. Equilibrium data were analyzed
using Langmuir and Freundlich isotherm models while the kinetics of the
process were examined using Lagergren Pseudo-first and second order, intra-
particle diffusion and Elovich kinetic models. Characterization of the acti-
vated carbon by Powder X-ray Diffraction (PXRD). The surface groups present
on the activated carbon surface were determined using the Fourier Transform
Infra-Red Spectroscopy (FTIR) analysis. Optimization studies were carried
out to determine the effects of pH, initial metal concentration, adsorbent do-
sage, contact time and adsorbent particle size on the Cr (VI) removal effi-
ciency. The results showed optimum Cr (VI) removal at pH 3, 10 mg/L con-
centration, 120 minutes of contact using 1000 - 1400 µm adsorbent particle
size at a dosage of 2.5 g/L. The adsorbent structure was found to be predomi-
nantly amorphous. The chromium removal efficiency of the adsorbent was
around 81.6%. Of the tested kinetic models, the pseudo-second order model
exhibited the best fit with the experimental data with an R
2
value of 0.9744.
This study clearly demonstrates the feasibility of using the nano-ZnO doped
scrap tyre derived activated carbon adsorbent for the remediation of chro-
mium (VI) polluted industrial wastewaters.
Keywords
Adsorption, Zinc Oxide Nanoparticles, Tire Granules, Hexavalent
Chromium, Tannery Effluent
How to cite this paper: Chigova, J. T., &
Mudono, S. (2022). Adsorption of Chro-
mium (VI) Using Nano-ZnO Doped Scrap
Tire-Derived Activated Carbon. Journal of
Geoscience and Environment Protection,
10, 121-135.
https://doi.org/10.4236/gep.2022.109008
Received: June 13, 2022
Accepted: September 24, 2022
Published: September 27, 2022
Copyright © 2022 by author(s) and
Scientific Research Publishing Inc.
This work is licensed under the Creative
Commons Attribution-NonCommercial
International License (CC BY-NC 4.0).
http://creativecommons.org/licenses/by-nc/4.0/
Open Access