Vol.:(0123456789)
Polymer Bulletin
https://doi.org/10.1007/s00289-020-03437-4
1 3
ORIGINAL PAPER
Modifcation of polysulfone ultrafltration membranes
using block copolymer Pluronic F127
Katsiaryna S. Burts
1
· Tatiana V. Plisko
1
· Alexandr V. Bildyukevich
1
·
Anastasia V. Penkova
2
· Svetlana A. Pratsenko
1
Received: 16 June 2020 / Revised: 4 October 2020 / Accepted: 20 October 2020
© Springer-Verlag GmbH Germany, part of Springer Nature 2020
Abstract
The efect of the addition of triblock copolymer polyethylene glycol (PEG)–poly-
propylene glycol (PPG)–polyethylene glycol (PEG) (Pluronic F127) and polyethyl-
ene glycol (PEG-4000, M
n
= 4000 g mol
−1
) to the polysulfone (PSF) casting solution
on the membrane structure and performance was studied. The phase state, viscosity
and turbidity of PSF solutions in N,N-dimethylacetamide (DMAc) with the addition
of block copolymer Pluronic F127 were investigated. It was found that 18–22 wt.%
PSF solutions in DMAc with Pluronic F127 content ≥ 5 wt.% feature a lower critical
solution temperature (LCST). Membrane structure was investigated using scanning
electron and atomic force microcopies. It was revealed that average pore size and
pore amount on the surface of the membrane selective layer increase and pore size
distribution becomes wider with an increase in Pluronic F127 content in the casting
solution. It was found that the average surface roughness parameters of the mem-
brane selective layer for PSF/Pluronic F127 membranes signifcantly exceed those
for PSF/PEG-4000 membranes. It was shown that the increase in the membrane fux
and the decrease in polyvinylpyrrolidone (PVP K-30, M
n
= 40,000 g mol
−1
) rejection
are a result of the addition of both Pluronic F127 and PEG-4000 into the casting
solution. It was revealed that PSF/Pluronic F127 membranes are characterized by
higher pressure resistance in ultrafltration process, a lower total fux decrease dur-
ing ultrafltration of bovine serum albumin solutions. The antifouling performance
of PSF/Pluronic F127 membranes was found to exceed signifcantly the antifouling
performance of PSF/PEG-4000 membranes.
Keywords Polysulfone · Pluronic F127 · Polyethylene glycol 4000 · Polymer
solution · Ultrafltration · Membrane modifcation · Fouling
* Tatiana V. Plisko
plisko.v.tatiana@gmail.com
Extended author information available on the last page of the article