Advances in Chemical Engineering and Science, 2021, 11, 105-140
https://www.scirp.org/journal/aces
ISSN Online: 2160-0406
ISSN Print: 2160-0392
DOI: 10.4236/aces.2021.111008 Jan. 29, 2021 105 Advances in Chemical Engineering and Science
Nanostage Alloying of Metals in Liquid Phase
Deblina Roy
1
, Tarasankar Pal
2
*
1
Department of Chemistry, National Institute of Technology, Rourkela, Odisha, India
2
Department of Chemical Sciences, Auckland Park Kingsway Campus, University of Johannesburg, Johannesburg, South Africa
Abstract
Alloying of metals is known from antiquity. Alloy making i.e., homogenizing
metals started in a “hit-or-miss” way. The 1
st
alloy from copper (Cu) and tin
(Sn) was produced around 2500 BC and from then Bronze Age began. Sub-
sequently iron (Fe) age started after the Bronze Age. Aluminium (Al) alloying
was discovered much later because pure Al could not be recovered easily even
though Al is the most abundant metal in the earth’s crust. Refining of Al is a
very difficult job because of its strong affinity towards oxygen. To ease alloy-
ing, melting points (mp) of the individual constituents and reactivity of metal
towards oxygen were the hurdles. Now understanding the thermodynamics of
metal mixing has paved alloying. Periodic properties of elements concerning
size, electronegativity, crystal structure, valency, lattice spacing, etc. are con-
sidered for alloying. In this feature article, more emphasis is given to
Hume-Rothery rules in which the necessary parameters for alloying have
been illustrated. Importantly standard electrode potential (E
0
) values, eutec-
tic, phase diagram, size-related strain in metals, etc. have been looked into in
the present discussion. One elegant example is Sn-Pb alloy, known as soft
solder. Soft solder was in use for many years to connect metals and in electric
circuitry. Low melting, flowability, and conductivity of soft solder had placed
Sn-Pb alloy a unique position in industries, laboratories and even in cottage
industries. However, toxic Pb volatilizes during soldering and hence soft
solder is banned almost in all countries. We felt the need for a viable alterna-
tive to obtain soldering material and then silver (Ag) based highly conduct-
ing, an eco-friendly alloy of Sn resulted in from a high boiling liquid. The
discovery engenders not only a new conducting soldering alloy but also a new
concept of melting metals together. Furthermore, new ideas of alloying have
been generalized at their nanostages from a suitable high boiling solvent.
Keywords
Alloy, Nanoparticles, Hume-Rothery Rules, Oriented Attachment, Ostwald
Ripening, Digestive Ripening, Galvanic Replacement Reaction, Kirkendall
How to cite this paper: Roy, D. and Pal, T.
(2021) Nanostage Alloying of Metals in Liquid
Phase. Advances in Chemical Engineering and
Science, 11, 105-140.
https://doi.org/10.4236/aces.2021.111008
Received: December 25, 2020
Accepted: January 26, 2021
Published: January 29, 2021
Copyright © 2021 by author(s) and
Scientific Research Publishing Inc.
This work is licensed under the Creative
Commons Attribution International
License (CC BY 4.0).
http://creativecommons.org/licenses/by/4.0/
Open Access