1. Introduction
Use of nanoparticles in numerous applications has
become a major area of interdisciplinary research in
recent times. The method of nanoparticle synthesis
is an important factor in determining the type of ap-
plication. The research, particularly on semiconduc-
tor nanoparticles is motivated by its possible uses in
various fields like nonlinear optics, solar cells, light-
emitting devices, electronics, biological labels, and
catalysis. The size-dependent mechanical, optical and
electronic properties are very much essential. When
a particle approaches the size of a few nanometers,
its diameter becomes equal to or less than the bulk
semiconductor exciton diameter (for cadmium sul-
fide it is 5–6 nm [1]), such that quantum confinement
of electron-hole pairs increase the band gap relative
to that in the bulk materials. Hence, the control of
particle size allows tuning of the band gap which
gives the desired above mentioned electronic and op-
tical properties. Reinforcement of inorganic nanopar-
ticles inside solid polymer matrices are attracting in-
creased attention because the combination of both
these materials provides a simple route to stable and
processable materials having properties of both com-
ponents incorporated in the matrix [1].
However, these composites normally cannot be re-dis-
solved while protecting the colloidal state of nanopar-
ticles. The single polymer molecule represents an im-
portant type because isolated nanocomposites based
on a single molecule can be obtained, which have very
desirable processing characteristics. Mainly, all the
applications which are based on single polymer mol-
ecule can be applied to the single molecule-nanopar-
ticle composites also. In most of these cases, the nano-
883
Influence of cadmium sulfide nanoparticles on structural
and electrical properties of polyvinyl alcohol films
J. Koteswararao
1
, R. Abhishek
1
, S. V. Satyanarayana
2
, G. M. Madhu
1*
, V. Venkatesham
1
1
Department of Chemical Engineering, M S Ramaiah Institute of Technology, 560054 Bangalore, Karnataka, India
2
Department of Chemical Engineering, Jawaharlal Nehru Technological University Anantapur, Anantapuramu – 515002,
Andhra Pradesh, India
Received 1 January 2016; accepted in revised form 20 June 2016
Abstract. Cadmium sulfide (CdS) nanoparticles have been synthesized by hydrothermal method and dispersed in poly vinyl
alcohol (PVA) matrix in varying amounts by weight. Subsequently, PVA/CdS nanocomposites have been synthesized with
the objective of investigating the effect of CdS nanoparticles on structural and electrical properties of PVA films. Structural
properties were analyzed by Fourier transform infrared spectroscopy (FTIR), X-ray diffraction (XRD) and scanning electron
microscopy (SEM) techniques. Differential scanning calorimetry (DSC) was used to investigate thermal properties of
PVA/CdS nanocomposites. Electrical properties were measured by using high frequency LCR meter and were found to be
strongly dependent on frequency and nano CdS content. Dielectric constant decreased with increase in frequency and with
increase in nanofiller concentration. AC conductivity and dielectric loss increased with frequency and decreased with increase
in nano CdS content.
Keywords: nanocomposites, cadmium sulfide, electrical properties, polyvinyl alcohol
eXPRESS Polymer Letters Vol.10, No.11 (2016) 883–894
Available online at www.expresspolymlett.com
DOI: 10.3144/expresspolymlett.2016.83
*
Corresponding author, e-mail: gmmadhu@gmail.com
© BME-PT