Vol.:(0123456789) 1 3
Arch Microbiol
DOI 10.1007/s00203-017-1438-2
ORIGINAL PAPER
A comparative analysis of tellurite detoxifcation by members
of the genus Shewanella
M. A. Valdivia‑González
1,2
· W. A. Díaz‑Vásquez
3
· D. Ruiz‑León
4
· A. A. Becerra
5
·
D. R. Aguayo
6
· J. M. Pérez‑Donoso
7
· C. C. Vásquez
1
Received: 28 July 2017 / Revised: 25 September 2017 / Accepted: 5 October 2017
© Springer-Verlag GmbH Germany 2017
transformation was associated with tellurium precipitation
as tellurium dioxide. In summary, this work highlights the
high tellurite reduction/detoxifcation ability exhibited by a
number of Shewanella species, which could represent the
starting point to develop friendly methods for the recovery
of elemental tellurium (or tellurium dioxide).
Keywords Shewanella · Tellurium · Tellurite · Antarctic ·
Heavy metals
Introduction
Tellurium and its derivatives have been widely used in the
oil-refning, electronic, optics, and sensor-generating indus-
tries (Sen et al. 2009; Tang et al. 2006; Turner et al. 2012;
Wang et al. 2011). Elemental tellurium (Te
0
) is a relatively
stable, water insoluble metalloid that displays low bioavail-
ability and toxicity. Conversely, the tellurium oxyanion, tel-
lurite (TeO
3
2−
), is water soluble and extremely harmful to
most microorganisms, mainly Gram-negative bacteria. For
instance, concentrations as low as 4 µM inhibit Escherichia
coli growth (Taylor 1999; Chasteen et al. 2009). However,
there are some Gram-negative bacteria isolated from Ant-
arctica that are tellurite resistant, including members of the
genus Acinetobacter and Psychrobacter (Arenas et al. 2014).
Although TeO
3
2−
can be toxic per se (Morales et al.
2017), the oxidative stress that is generated during tellurite
reduction to elemental tellurium (Te
0
) under aerobic condi-
tions seems to be the main responsible for tellurite toxicity
(Chasteen et al. 2009; Pérez et al. 2007). Under anaero-
bic conditions, where reactive oxygen species (ROS) are
not generated (Imlay 2013), TeO
3
2−
can also kill E. coli,
although the toxicant’s MIC is 10-fold higher (Tantaleán
et al. 2003).
Abstract The increasing industrial utilization of tellu-
rium has resulted in an important environmental pollution
with the soluble, extremely toxic oxyanion tellurite. In this
context, the use of microorganisms for detoxifying tellur-
ite or tellurium biorecovery has gained great interest. The
ability of diferent Shewanella strains to reduce tellurite to
elemental tellurium was assessed; the results showed that
the reduction process is dependent on electron transport
and the ∆pH gradient. While S. baltica OS155 showed the
highest tellurite resistance, S. putrefaciens was the most ef-
cient in reducing tellurite. Moreover, pH-dependent tellurite
Communicated by Jorge Membrillo-Hernández.
Electronic supplementary material The online version of this
article (doi:10.1007/s00203-017-1438-2) contains supplementary
material, which is available to authorized users.
* C. C. Vásquez
claudio.vasquez@usach.cl
1
Laboratorio de Microbiología Molecular, Departamento de
Biología, Facultad de Química y Biología, Universidad de
Santiago de Chile, Avenida Libertador Bernardo O’Higgins
#3363. Estación Central, Santiago, Chile
2
Facultad de Ciencias de la Educación, Universidad Central
de Chile, Santiago, Chile
3
Facultad de Ciencias de la Salud, Universidad San Sebastián,
Providencia, Chile
4
Departamento de Química de los Materiales, Universidad de
Santiago de Chile, Santiago, Chile
5
Facultad de Salud, Deporte y Recreación, Universidad
Bernardo O’Higgins, Santiago, Chile
6
Molecular Biophysics and Bionformatics Group, Universidad
Andrés Bello, Santiago, Chile
7
BioNanotechnology and Microbiology Laboratory,
Universidad Andrés Bello, Santiago, Chile