© 2015 N.R. Caetano et al., licensee De Gruyter Open.
This work is licensed under the Creative Commons Attribution-NonCommercial-NoDerivs 3.0 License.
Open Eng. 2015; 5:213–219
Research Article Open Access
Nattan R. Caetano*, Diego Soares, Roger P. Nunes, Fernando M. Pereira, Paulo Smith
Schneider, Horácio A. Vielmo, and Flávio Tadeu van der Laan
A comparison of experimental results of soot production in
laminar premixed flames
Abstract: Soot emission has been the focus of numerous
studies due to the numerous applications in industry, as
well as the harmful effects caused to the environment.
Thus, the purpose of this work is to analyze the soot for-
mation in a flat flame burner using premixed compressed
natural gas and air, where these quasi-adiabatic flames
have one-dimensional characteristics. The measurements
were performed applying the light extinction technique.
The air/fuel equivalence ratio was varied to assess the soot
volume fractions for different flame configurations. Soot
production along the flame was also analyzed by measure-
ments at different heights in relation to the burner surface.
Results indicate that soot volume fraction increases with
the equivalence ratio. The higher regions of the flame were
analyzed in order to map the soot distribution on these
flames. The results are incorporated into the experimen-
tal database for measurement techniques calibration and
for computational models validation of soot formation in
methane premixed laminar flames, where the equivalence
ratio ranging from 1.5 up to 8.
Keywords: soot volume fraction; light extinction tech-
nique; premixed flat flame
DOI 10.1515/eng-2015-0016
Received September 05, 2014; accepted January 20, 2015
1 Introduction
Soot can be defined as the solid particulate matter pro-
duced during combustion [1]. The process of formation is
*Corresponding Author: Nattan R. Caetano: Dept of Mechanical
Engineering, Federal University of Rio Grande do Sul (UFRGS), Porto
Alegre, RS, Brazil, E-mail: nattan@ufrgs.br
Diego Soares, Roger P. Nunes, Fernando M. Pereira, Paulo Smith
Schneider, Horácio A. Vielmo, Flávio Tadeu van der Laan: Dept
of Mechanical Engineering, Federal University of Rio Grande do Sul
(UFRGS), Porto Alegre, RS, Brazil
based in the conversion and agglomeration of the carbon
atoms contained in the hydrocarbon fuel molecules. The
formation of soot is not completely understood due to the
complexity and velocity of this transformation. Soot is of
great interest in engineering, insofar as its formation in-
creases the radiated heat transfer, which can be a positive
to the considered system. The excessive presence of partic-
ulate in diesel engines is, an example, where soot is harm-
ful. These particles resulted from an inadequate combus-
tion process can become logged in the seat of valves, pre-
venting a proper seal in the combustion chamber and lead-
ing to a loss of compression in the cylinder. Another exam-
ple is gas turbines, where the presence of soot affects the
life of the blades due to abrasion for the contact.
The emission of this type of particulate matter into the
atmosphere causes great harm to the environment, since
there is a significant deterioration in air quality. Also, in-
duce respiratory problems in humans and is associated
with the occurrence of cancer. On the other hand, in in-
dustrial heating equipment such as a boiler, the presence
of soot increases the heat exchange by radiation from the
flame to the system walls, whereas the solid material re-
sulting from the process absorbs and emits radiation at a
wide range in the wavelengths spectrum [2]. Thus, where
a large and uniform heat transfer is required, the presence
of soot in combustion is purposely induced.
To control the emission of soot in real combustion sys-
tems, it is necessary to understand the soot formation and
oxidation mechanisms. The basis of knowledge is the de-
velopment of models that can predict the particulate mat-
ter formation, and the validation of these models requires
information about the soot volume fraction. In this way,
optical techniques are generally employed to perform the
measurement of these quantities due the non- intrusive
probing.
The necessity for such information in the study of com-
bustion was what motivated the present work, which was
developed in order to produce significant results for future
calibration of measurement techniques and validation of
theoretical models in this subject. Hence, the main objec-
tive of this study is to analyze the production of soot in pre-
mixed laminar flat flames of natural gas and air, measur-