Xylitol Production from Wood Hydrolyzates 119
Applied Biochemistry and Biotechnology Vol. 81, 1999
Copyright © 1999 by Humana Press Inc.
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119
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Xylitol Production from Wood Hydrolyzates
by Entrapped Debaryomyces hansenii
and Candida guilliermondii Cells
JOSE MANUEL DOMÍNGUEZ,*
,1
JOSE MANUEL CRUZ,
1
ENRIQUE ROCA,
2
HERMINIA DOMÍNGUEZ,
1
AND JUAN CARLOS PARAJÓ
1
1
Chemical Engineering Department,
University of Vigo (Campus Ourense), 32004 Ourense, Spain,
E-mail: jmanuel@uvigo.es;
2
Chemical Engineering Department,
Instituto de Investigaciones Tecnológicas,
University of Santiago de Compostela (Campus Lugo), 27002-Lugo, Spain
Received August 28, 1998; Revised December 23, 1998; Accepted December 30, 1998
Abstract
Debaryomyces hansenii cells were entrapped in Ca-alginate beads and used
for producing xylitol from wood hydrolyzates. Batch experiments showed
that bioconversion was severely hindered when Ca-alginate beads were
hardened with Al
3+
solutions. As an alternative to Al
3+
hardening, the
improvements in both mechanical stability of bioparticles and fermenting
ability of the immobilized system derived from using increased concentra-
tions of sodium alginate were assessed. The best results were obtained using
a 4% (w/v) Na-alginate solution in the gelification step. This concentration
was selected to perform continuous fermentations in a packed-bed reactor
using raw or charcoal-treated hydrolyzates (15.5 g of xylose/L) with two
different yeasts: Candida guilliermondii and Debaryomyces hansenii. With a final
cell concentration of about 50 g of cells/L (0.075 g of cells/g of beads), the
volumetric productivities reached with these yeasts in media made from
charcoal-treated hydrolyzates were 0.58 and 0.91 g/L·h, respectively.
Index Entries: Ca-alginate; Candida guilliermondii; Debaryomyces hansenii;
hemicellulose hydrolyzate; xylitol.
Introduction
Xylitol, a five-carbon polyol with high sweetening power, is tolerated
by diabetics, has anticariogenic properties, and has been recommended for