Vol.:(0123456789) 1 3
Innovative Infrastructure Solutions (2020) 5:95
https://doi.org/10.1007/s41062-020-00342-7
STATE-OF-THE-ART PAPER
Possible efects and reactions between leachate and diferent clay
material types
I. A. Oyediran
1
· D. A. Olalusi
1
· M. T. Jimoh
2
Received: 18 April 2020 / Accepted: 14 July 2020
© Springer Nature Switzerland AG 2020
Abstract
Interactions between landfll leachate and some clayey soils were investigated to elucidate their possible efects and reactions
and the extent to which the chemical composition of landfll leachate infuences the chemical and mineralogical properties
of the soils upon leachate contact. Physicochemical properties of landfll leachate was obtained while the clay mineralogy,
major and minor oxides composition, pH, cation exchange capacity (CEC), carbonate content and total organic carbon of
Shale (Sedimentary), Migmatite gneiss and Quartzite (Basement Complex)-derived clayey soils after three-weeks saturation
with leachate were determined. Dark brown colour and malodorous smell of landfll leachate is linked to high concentration
of dissolved organic substances in the leachate composition while high leachate pH indicates an old and stabilized leachate
with its temperature impacting the bacterial growth and chemical reaction. Signifcant changes were observed in both chem-
istry and mineralogy of the clays after leachate contact with observed appearance of Illite in the migmatite gneiss-derived
clayey soil, an indication of mineralogical changes caused by ionic solutions. Enrichment of Ca, SiO
2
and Cl; in addition
to increased CEC for all the soils is generally noticed. Furthermore, leachate contact resulted in modifcation of Basement
Complex-derived soils from acidic to alkaline soils while the sedimentary terrain-derived soils retained its alkaline pH
nature. Hence, alteration in mineralogical and chemical properties observed in the diferent derived clayey soils is a func-
tion of the leachate composition, sorptive capacity of the soils, parent material and especially the inherent reactions upon
leachate contact.
Keywords Reactions · Landfll leachate · Alteration · Signifcant changes
Introduction
Landfll leachate formed from urban solid waste is com-
monly contaminated and contains multifaceted wastewater
[1, 2]. The generation of leachate is as a result of percola-
tion of precipitation via open landfll coupled by means of
any disposed liquid wastes, which results in the withdrawal
of water soluble compounds and particulate material of the
wastes [3]. The distinctiveness of leachate are greatly unpre-
dictable depending on the waste composition, amount of pre-
cipitation, site hydrology, waste compaction, cover design,
sampling procedures and leachate—soil interaction, others
are landfll design and operation [4, 5]. Clay soils have over
the years become the preferred barrier and liner material
commonly used in engineered waste disposal systems in
order to curtail leachate movement and protect the underly-
ing soils and aquifers. Rowe et al. [6] and Rowe [7] opined
that these natural materials have become the veritable option
for use particularly because of their availability, low cost
for a relative thick lining, long life and attenuating ability.
However, the reactions, which take place between these most
preferred barrier option (clayey soils) and natural leachate
as opposed to synthetic leachate (or in some cases water)
have not been well documented. In addition, data on the
responses of the diferent clay soils which possess diverse
mineralogical composition and chemistry particularly as it
relates to soil properties and associated reactions is scanty.
More importantly, an examination of the compatibility of
the clays with waste leachate is required since Shackelford
and Jeferis [8] stipulated that one of the fundamental design
* I. A. Oyediran
oyediranibrahim2012@gmail.com;
oyediranibrahim@yahoo.com
1
Department of Geology, Faculty of Science, University
of Ibadan, Ibadan, Nigeria
2
Department of Earth Science, Ladoke Akintola University
of Technology, Ogbomoso, Nigeria