© 2007 Society of Vacuum Coaters 505/856-7188 59
50th Annual Technical Conference Proceedings (2007) ISSN 0737-5921
ABSTRACT
A novel hollow cathode plasma immersion ion processing
method is developed and used to deposit silicon containing
diamond like carbon (DLC-Si) coatings inside a one foot
long 304 stainless steel (304SS) pipe with 1.5 inch diameter
and 0.065 inch wall thickness. A multilayer DLC-Si coating
structure was deposited using a combination of carbon and
silicon precursors starting with silicon-rich adhesion layer.
Result shows that the interface between the substrate and ad-
hesion layer contains silicon as well as substrate constituents.
Within this interface, isolated crystalline structure embed-
ded within amorphous matrix was present while deposited
DLC-Si coating is amorphous. Data show that the layered
DLC-Si coating structure not only improves the friction and
wear performance of the internal surface of 304SS pipe but
also improves the corrosion resistance. The hardness and
modulus of the coating was measured at 19GPa and 138GPa,
respectively. It is suggested that this new technology enables
wide spread use of DLC based coatings to increase component
life in applications where the internal surface of pipes are
exposed to corrosive and abrasive environments especially
in oil and gas industry.
INTRODUCTION
Diamond-like carbon (DLC) coatings have excellent properties
such as high wear resistance, very low friction coeffcient and
high corrosion resistance [1-3]. Because of these excellent
properties, DLC coatings have attracted great attention for
use in various applications in industries such as oil and gas,
semiconductor, medical and automotive. In the oil and gas
industry, DLC coatings are especially expected to improve
the tribological and corrosion performance of components
that experience extreme environments. For piping or tubing
that delivers corrosive material, obviously the interior surface
that is in contact with the corrosive material is the surface
that must be coated. There are several methods available to
deposit DLC based protective coatings at the outer surface
of component such as chemical vapor deposition (CVD),
physical vapor deposition (PVD), electroplating, fame spray
and sol-gel. However, coating internal surfaces remains a
challenge especially for large aspect ratio (length to diameter
ratio) components and very limited information is available
in literature.
Investigation of DLC-Si Film Deposited Inside a 304SS Pipe Using a Novel Hollow
Cathode Plasma Immersion Ion Processing Method
T. Casserly, K. Boinapally, M. Oppus, D. Upadhyaya, B. Boardman, and A. Tudhope,
Sub-One Technology, Inc., Pleasanton, CA
Various methods of coating the interior surfaces of tubes have
been attempted whereby the source material to be coated is
inserted into the tube and then sputtered or arced off onto the
tube [4,5]. It is reported that a chamber based plasma assisted
chemical vapor deposition (PACVD) can be used to deposit
coating on small aspect ratio components such as small hollow
pins (15mm x 100mm) with a thin layer of DLC-Si [6,7]. In
contrast to the work presented here where, these processes
use a separate chamber and have a much lower deposition
rates, so that much thicker flms, needed for corrosion and
abrasion resistance, can not be deposited.
This article demonstrates the potential of a new technology to
deposit multilayer DLC-Si based flm on internal surfaces of
pipes and presents microstructural, corrosion and mechanical
performance data.
EXPERIMENTAL
Coating Deposition
A novel hollow cathode plasma immersion ion processing
method is developed and used to deposit silicon containing
diamond like carbon (DLC-Si) flms onto the internal surface
of a 304SS pipe. This method takes advantage of plasma ion
immersion and hollow cathode plasma generated within the
pipe itself allowing decomposition of precursor gases and
subsequent deposition of DLC-Si based flms. As seen in Figure
1, this is done by negatively pulse biasing the pipe, which acts
as the cathode, with anodes attached at the ends. A gaseous
precursor is introduced and ionized causing a coating to be
deposited on the pipe, with by-products pumped out [8].
Figure 1: Diagram of Process Set-up [8].