Blue-light emission from GaN self-assembled quantum dots due to giant piezoelectric effect F. Widmann, J. Simon, B. Daudin, G. Feuillet, J. L. Rouvie ` re, and N. T. Pelekanos De ´partement de Recherche Fondamentale sur la Matie `re Condense ´e, CEA/Grenoble, SPMM,* 17 rue des Martyrs, 38054 Grenoble Cedex 9, France G. Fishman Laboratoire de Spectrome ´trie Physique, UMR C5588, Universite ´ Joseph Fourier, Grenoble 1, CNRS, Boı ˆte Postale 87, 38402 St. Martin d’He `res Cedex, France Received 27 July 1998; revised manuscript received 25 September 1998 It is shown that the optical properties of GaN quantum dots with the wurtzite structure result from a balance between confinement and piezoelectric effects. In ‘‘large’’ quantum dots with an average height and diameter of 4.1 and 17 nm, respectively, the photoluminescence peak is centered at 2.95 eV, nearly 0.5 eV below the bulk GaN band gap. We attribute this enormous redshift to a giant 5.5 MV/cm piezoelectric field present in the dots, in agreement with theoretical calculations. S0163-18299851248-9 The current interest in low-dimensional heterostructures mainly relies on the possibility of achieving high-quality de- vices, due to the optical and electronic properties which are expected to result from one-dimensional 1Dquantum wiresor 0D quantum dotscarrier confinement. In particu- lar, it has been theoretically predicted that the realization of light-emitting diodes LEDsor laser diodes LDswith quantum dots QDsin the active layer would lead to im- proved optical characteristics, such as low threshold current and weak temperature dependence of the threshold current. 1 However, the practical observation of 0D confinement ef- fects requires the use of objects with typical sizes in the 10 nm range. The first pioneering works in the field used almost exclusively lithographic patterning of QDs. Nevertheless, this approach is practically abandoned today because of the damage that lithographic processing causes on the lateral QD walls, seriously degrading the optical properties when the QD dimension becomes of the order of 10 nm. By contrast, self-organization resulting from the Stranski-Krastanov growth mode has proven to be very successful in achieving nanostructures with excellent 0D optical properties. In this growth mode, deposition of a strained 2D wetting layer is followed by elastic relaxation through 3D islanding which results in free surface formation. 2 It has been observed for various materials grown under compressive stress, such as InAs on GaAs, 3 InP on Ga x In 1 -x P, 4 or SiGe on Si, 5 opening the way for achievement of lasers based on self-organized In x Ga 1 -x As/GaAs Refs. 6 and 7and InAs/GaAs Refs. 8 and 9QDs. Concerning III-V nitrides, the present day blue LEDs and LDs consist of stacking of 2D layers with appropriate composition. 10 Despite the successful operation of such LEDs and LDs it is still a current challenge to improve char- acteristics such as device life time or current threshold. In particular, the insertion of GaN QDs in the active layer ap- pears particularly promising, following the experimental demonstration that nitrides grown under compression by mo- lecular beam epitaxy MBEexhibit a Stranski-Krastanov growth mode 11 and that the size of the 3D islands is suffi- ciently small to allow them to behave as QDs. 12,13 Alterna- tively, it has also been demonstrated that 3D growth of GaN could be induced in metalorganic chemical vapor deposition MOCVDby using Si as an antisurfactant. 14,15 Whatever the growth technique, i.e., MBE or MOCVD, the QDs exhibit the wurtzite structure, with the 0001axis parallel to the growth direction. Thus, as a consequence of the noncentrosymmetry of the wurtzite structure, piezoelec- tric effects are expected to be present and to govern the op- tical properties of the dots to a certain extent, due to the huge piezoelectric constant values which are one of the most fas- cinating aspects of nitrides. Actually, for fully strained GaN on AlN =2.5%piezo- electric fields as high as several MV/cm are expected. 16–18 These values are more than one order of magnitude larger than the piezoelectric fields that can be found in zincblende semiconductors for the same amount of strain. 19 Neverthe- less, the role of these giant piezoelectric fields on the optical properties of nitride nanostructures has only recently started to be assessed. For example, large piezoelectric field-induced redshifts in photoluminescence PLspectra of GaN/Al x Ga 1 -x N quantum wells have been reported lately. 20,21 However, the role of dislocations, interdiffusion, and re- sidual impurities in compensating the piezoelectric field in those systems needs to be further investigated. From this point of view, GaN quantum dots are of special interest as they are fully strained in the AlN matrix and exhibit almost no interdiffusion. Although it has been observed 12 that the threading dislocations existing in the AlN buffer and origi- nating from the sapphire/AlN interface act often as nucle- ation centers for the QDs, their far inferior density 10 10 cm -2 compared to the QDs which are in the 10 11 cm -2 range explains how the vast majority of the QDs are dislocation-free. This is further supported by the obser- vation of intense and temperature-independent QD photoluminescence. 12 The samples used in the present study were grown on 0001sapphire substrate. After the nitridation step of the sapphire, a low-temperature AlN layer, about 15 nm thick, was deposited followed by the growth of a 1.5-m-thick RAPID COMMUNICATIONS PHYSICAL REVIEW B 15 DECEMBER 1998-II VOLUME 58, NUMBER 24 PRB 58 0163-1829/98/5824/159894/$15.00 R15 989 ©1998 The American Physical Society