Physica A 177 (1991) 495-504
North-Holland
Sum rules for interface Hamiltonians
Lev V. Mikheev and John D. Weeks
Institute for Physical,Science and Technology, University of Maryland, College Park, MD 20742,
USA
We derive exact identities for a general class of interface Hamiltonians describing wetting tran-
sitions that relate force fluctuations to interface fluctuations and the surface tension. These sum
rules are analogous to the Triezenbeg, Zwanzig and Wertheim formulas for the surface tension
derived using the theory of inhomogeneous fluids. Relations between these two approaches are
discussed. Our sum rules are consistent with the scaling theory of wetting transitions.
1. Introduction
There are two basic strategies used to study properties of an inhomogeneous d-
dimensional system containing interfaces and boundaries or walls. The most straight-
forward approach in principle is to use the modern theory of inhomogeneous fluids ~1
[ 2 ] to determine thermodynamic properties and density correlation functions for the
full d-dimensional system as a function of an external field ¢ and the interparticle
interactions. In practice, approximations are often made whose errors are difficult to
assess. Thus it is of particular interest to study certain exact sum rules: equilibrium
identities relating a macroscopic thermodynamic property such as the surface tension
to integrals over correlation functions. Relations between exponents describing inter-
face phase transitions can often be derived by combining a scaling ansatz for the cor-
relation functions along with an appropriate sum rule. Henderson [2,3] has shown
the utility of such an approach for a variety of problems, including in particular wet-
ting transitions [ 3 ], which will be our main focus in this article.
A second, more phenomenological but often conceptually simpler, approach is to
study the properties of a d' =- d- 1 construct, the interface Hamiltonian #2 [ 5--8 ]. At
wavelengths long compared to the bulk correlation length, the important remaining
degrees of freedom can often be described in terms of interfaces, their effective inter-
actions and their fluctuations, as described by the appropriate interface Hamiltonian.
This viewpoint is very general, and forms the basis for renormalization group studies
of interfacial phenomena [4,6-8]. However, the relationship between the effective
~ For a general review, see ref. [ 1].
~z For a general review, see ref. [4].
0378-4371/91/$03.50 © 1991 - Elsevier Science Publishers B.V. (North-Holland)