321
ISSN 0021-3640, JETP Letters, 2016, Vol. 103, No. 5, pp. 321–327. © Pleiades Publishing, Inc., 2016.
Effect of a Magnetic Field on the Intermediate Phase in Mn
1 – x
Fe
x
Si:
Spin-Liquid versus Fluctuations Scenario
1
S. V. Demishev
a, b,
*, I. I. Lobanova
a, b
, A. V. Bogach
a
, V. V. Glushkov
a, b
, V. Yu. Ivanov
a
,
T. V. Ischenko
a
, N. A. Samarin
a
, N. E. Sluchanko
a
, S. Gabani
c
, E. Čižmár
d
,
K. Flachbart
c
, N. M. Chubova
e
, V. A. Dyadkin
e, f
, and S. V. Grigoriev
e
a
Prokhorov General Physics Institute, Russian Academy of Sciences, Moscow, 119991 Russia
b
Moscow Institute of Physics and Technology (State University), Dolgoprudnyi, Moscow region, 141700 Russia
c
Institute of Experimental Physics, Slovak Academy of Sciences, 040 01 Košice, Slovak Republic
d
P.J. Šafárik University in Košice, SK-04001 Košice, Slovak Republic
e
Petersburg Nuclear Physics Institute, Gatchina, 188300 Russia
f
Swiss–Norwegian Beamlines at the European Synchrotron Radiation Facility, 38000 Grenoble, France
* e-mail: demis@lt.gpi.ru
Received December 1, 2015; in final form, January 18, 2016
We report results of the magnetic field influence on the chiral spin liquid state in Mn
1 – x
Fe
x
Si single crystal
with iron content x = 0.108 in proximity of a hidden quantum critical point. The use of small angle neutron
scattering data together with magnetic susceptibility measurements down to 0.4 K and precise magnetoresis-
tance measurements in the temperature range 2–20 K in magnetic field up to 5 T allowed us to construct the
magnetic phase diagram of this compound in which at low magnetic fields B < 0.15 T an intermediate phase
with short-range magnetic order exists in a wide temperature range 0.62 K < T < 9.1 K. It was found that the
increase in magnetic field first results in the suppression of a transition to the spiral phase with long-range
magnetic order at very low temperatures, and then induces a transition of the intermediate phase to a spin-
polarized (ferromagnetic) phase with lowering temperature. The temperature of this transition T
SP
increases
with magnetic field logarithmically, T
SP
~ log(B), and results in formation of a singular point on the magnetic
phase diagram located at T ~ 8.5 K and B ~ 3.5 T, which may be either a triple or a critical point. The possible
spin-liquid nature of the intermediate phase is discussed.
DOI: 10.1134/S0021364016050027
1. Spiral magnets Mn
1 – x
Fe
x
Si are characterized by
presence of unusual magnetic phases, which are inter-
mediate between common paramagnetic phase (PM)
and spiral magnet (SM) phase with a long-range mag-
netic order [1–4]. These intermediate phases (IP) may
be detected either on B–T [1, 3] or on T –x [1, 2, 4]
magnetic phase diagrams. Several theoretical studies
also predict phases with an intermediate magnetic
order for MnSi based solids [5, 6]. These results may
be qualitatively understood following experimentally
supported similarity between spiral magnets and cho-
lesteric liquid crystals [7], in which the considered
intermediate phases appear as a magnetic analog of
the blue fog phases [5, 7, 8]. The IP are also referred as
spin liquid (or chiral spin liquid) states due to straight-
forward analogy from general physics, where the para-
magnetic phase, spiral phase with long-range order
(LRO) and intermediate phase may be considered as
magnetic replicas of the common gas, solid and liquid
phases [5]. Nevertheless, sometimes the aforemen-
tioned description of the intermediate magnetic
phases is disputed, and these specific states are treated
as regions of pronounced magnetic f luctuations in the
phase diagram [9]. In any case, these specific phases
are of magnetic nature and thus may be affected by
external magnetic field; however, the influence of
magnetic field on the phases with intermediate mag-
netic order has not yet been systematically studied. At
the same time, an analogy with liquid crystals suggests
that the external field may noticeably change the cor-
responding phase diagram [8].
The aim of this work is to study experimentally the
influence of magnetic field on the intermediate mag-
netic phase in Mn
1 – x
Fe
x
Si developing in proximity to
the hidden quantum critical point at x* ~ 0.11 [4]. For
this iron concentration the transition to the SM phase
with long-range magnetic order is expected to be sup-
pressed and an intermediate magnetic phase may be
observed at temperatures below T
s
~ 9–10 K in zero
magnetic field, so that the quantum phase transition
1
The article is published in the original.
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