Introduction
Antipyrine (2,3-dimethyl-1-phenyl-3-pyrazolin-5-
one) and its derivatives possess a wide variety of po-
tentially useful application, including biological
[1, 2], clinical [3] and pharmacological areas [4].
They are also used as antipyretic, analgesic and
anti-rheumatic materials [5–8]. Antipyrines have also
been used as analytical reagents in determination of
some metal ions [9]. Follow up literature indicate that
considerable study has been devoted to Schiff bases
and azo containing ligands derived from either
4-amino- or 4-formylantipyrine [10–12]. However,
all the reported studies on this type of compounds are
concerning with synthesis, structure and properties.
However, comparatively less is known regarding
their thermal behaviour. The present study extends to
synthesis, characterization and thermal behaviour
studies of UO
2
(VI), Sn(IV), Th(IV) and Li(I) com-
plexes with 4-azomalononitrile antipyrine (L).
Experimental
Reagent grade chemicals were used without further
purification. The ligand 4-azomalononitrile anti-
pyrine (Scheme 1) was prepared and characterized as
described [13].
The metal complexes were prepared by stirring
magnetically at ca. 60°C an ethanolic solution (0.002
mol) of a metal salt of UO
2
(VI) chloride, nitrate, ace-
tate, Sn(IV) diphenyl chloride, Sn(IV) chloride,
Th(IV) nitrate or Li(I) chlorate (VII) with (0.002 or
0.004 mol) 4-azomalononitrile antipyrine (L) in
ca. 50 mL EtOH for periods of 5 h or more. The re-
sulting solids were filtered off, washed several times
with EtOH and dried under vacuum over P
4
O
10
. Ele-
mental analysis (C, H and Cl) were performed by the
Microanalytical unit of the University of Cairo,
Egypt. Metal analyses were estimated using standard
methods. IR spectra in the 4000–200 cm
–1
range were
performed as KBr discs using a PerkinElmer 1430 re-
cording spectrophotometer.
1
H NMR spectra were re-
corded in DMSO-d
6
using a 300 MHz Varian NMR
spectrometer. The molar conductivity measurements
were made in DMF solutions (10
–3
M) using a
Tacussel conductometer type CD6N. Thermal
analyses (DTA/TG) were carried out under N
2
atmo-
sphere using a Schimadzu DT-50 thermal analyzer at
a heating rate of 10°C min
–1
in the temperature range
25–800°C using platinum crucibles.
1388–6150/$20.00 Akadémiai Kiadó, Budapest, Hungary
© 2008 Akadémiai Kiadó, Budapest
UO
2
(VI), Sn(IV), Th(IV) AND Li(I) COMPLEXES OF 4-AZOMALONO-
NITRILE ANTIPYRINE
Synthesis, characterization and thermal studies
H. A. El-Boraey
1*
, F. A. El-Saied
1
and S. A. Aly
2
1
Department of Chemistry, Faculty of Science, El-Menoufia University, Shebin El-Kom, Egypt
2
Department of Chemistry, Genetic Engineering and Biotechnology Research Institute, El-Menoufia University, Sadat City, Egypt
UO
2
(VI), Sn(IV), Th(IV) and Li(I) complexes of 4-azomalononitrile antipyrine (L) have been isolated and characterized based on
IR spectra,
1
H NMR, elemental analyses, molar conductance and thermal analysis (DTA/TG). The study revealed that the ligand be-
haves as a neutral bidentate one and coordination takes place via the carbonyl atom of pyrazolone ring >C=O and the azomethine ni-
trogen >C=N. The thermal stability of the metal complexes were investigated by thermogravimetry (TG), differential thermal anal-
ysis (DTA) techniques and infrared spectra, and correlated to their structure. The thermal study revealed that Th(IV) complexes
show lower thermal stability than both UO
2
(VI) and Sn(IV) complexes.
Keywords: complexes, conductivity, IR, synthesis, thermal analysis (DTA/TG)
Scheme 1
* Author for correspondence: helboraey@yahoo.com
Springer, Dordrecht, The Netherlands
Journal of Thermal Analysis and Calorimetry, Vol. 96 (2009) 2, 599–606