33
Mater. Res. Soc. Symp. Proc. Vol. 1371 © 2012 Materials Research Society
DOI: 10.1557/opl.2012.
VLS Synthesis and Characterization of SnO
2
Nanowires
Dulce N. Castillo, Tomás D. Becerril, Enrique R. Andrés, Héctor J. Santiesteban and Godofredo
G. Salgado.
Posgrado en Dispositivos Semiconductores, Benemérita Universidad Autónoma de Puebla, Av.
14 Sur y San Claudio s/n, Ciudad Universitaria, C.P.72570, Puebla, Pue., México.
ABSTRACT
We have synthesized core-shell 1D nanostructures by the Vapor-Liquid-Solid (VLS)
mechanism. Gold (Au) was used as a catalyst and tin oxide (SnO) powder as a precursor; the
growth temperature was of 600 °C. These structures were characterized by XRD, SEM, TEM,
EDS, and PL. The nanowires have an average diameter of 20 nm and their lengths are of tens of
micrometers; the core is tin dioxide (SnO
2
) with the tetragonal rutile structure and it has an
average diameter of 12 nm; the shell is amorphous Sn of 8 nm average thickness.
Photoluminescence measurements show a broad band in the 400-800 nm range. On the same
growth process, SnO
2
nanoparticles and a mixture of SnO
2
rods and wires were also obtained, at
400 °C and 800 °C, respectively.
INTRODUCTION
SnO
2
is an n-type-semiconductor metal oxide whose bulk properties are: wide bandgap of
3.6 eV (at 300 K), low resistivity (10
-4
to 10
-6
ȍ-cm), high achievable carrier concentration (up
to 6x10
20
cm
-3
), high optical transparency in the visible range, and chemical and structural
stability [1,2].
Nanomaterials have mechanical, chemical, thermal, electrical, and optical properties
different from those of their bulk counterparts due to the enhanced surface-volume ratio and
possible quantum confinement effects [3-5].
Therefore, SnO
2
1D nanostructures are very interesting due to the various applications of
SnO
2
in optoelectronic and electronic devices and as transparent conductive electrodes, catalysts,
anode materials for lithium-ion batteries, and gas sensors. It is used also in field effect transistors
and it has been shown to act as a sub-wavelength waveguide [4, 6-10].
EXPERIMENTAL
Core-shell nanowires were synthesized by the VLS mechanism [11]. The growth process
was carried out inside a horizontal reactor (a quartz tube closed at one end) which was inserted
into a quartz-tube furnace. Gold, deposited as an ~150 nm thick film over Si substrates in a
vacuum evaporator, was used as a catalyst and powder SnO (99.9%) as a precursor. Three
substrates and an alumina crucible containing the SnO powder precursor were placed inside the
reactor in such a way that, when the reactor is inserted into the furnace quartz tube, each
substrate lies in a different temperature zone of the furnace and so does the precursor powder
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