Available online at www.sciencedirect.com
ScienceDirect
Materials Today: Proceedings 22 (2020) 1669–1675 www.materialstoday.com/proceedings
2214-7853 © 2019 Elsevier Ltd. All rights reserved.
Peer-review under responsibility of the scientific committee of the 2nd International Conference on Materials Manufacturing and Modelling,
ICMMM – 2019.
ICMMM 2019
Process parameter effects on particle size reduction of sol-gel
synthesized silica nanoparticles
Tankeshwar Prasad
a*
, Sudipta Halder
a
, S. S. Dhar
b
a
Department of Mechanical Engineering, National Institute of Technology Silchar, Silchar-788010, Assam, India
b
Department of Chemistry, National Institute of Technology Silchar, Silchar, Assam, 788010, India
Abstract
In present study, SiO
2
nanoparticle was prepared using sol-gel method. Tetraethyl orthosilicate (TEOS) was chosen as a silica
precursor, ethanol as a solvent, water as co-solvent and ammonia as a catalyst. The effects of most influencing process
parameters molar ratio (0.5, 1 and 2) of tetra-(ethyl)-orthosilicate (TEOS) to ammonia (NH
3
) with respect to particle size
variation was investigated experimentally in detail. The size of SiO
2
particles was controlled by tuning the NH
3
concentration
with respect to TEOS. Scanning electron microcopy (SEM) studies were performed for understanding the size of SiO
2
nanoparticles while surface functional groups was determine by Fourier transform infrared (FTIR). The amorphous phase and
purity of particles was identified by X-ray diffraction (X-RD) and energy dispersive spectroscopy (EDS) respectively. This work
demonstrates the molar ratio variation had the noticeable effect on particle size reduction of SiO
2
particles. it was found that the
particle size decreases with increases of NH
3
concentration with respect to TEOS (molar ratio = 1) and found lowest particle size
of 40 nm (TEOS: NH
3
) with fixed amount of TEOS, ethanol, water and reaction time.
© 2019 Elsevier Ltd. All rights reserved.
Peer-review under responsibility of the scientific committee of the 2nd International Conference on Materials Manufacturing and
Modelling, ICMMM – 2019.
Keywords: silica particles, sol-gel method, ammonia concentration, SEM, particle size;
1. Introduction
With increasing demand of nanomaterials, SiO
2
is the most important ceramic material which is extensively used
in chemical and advance polymer industries owing nanosized of particle with large surface area [1]. The quality of
these particles is mostly dependent on the geometrical shape, size and surface chemistry of SiO
2
particles [2].
*
Tankeshwar Prasad. Tel.: +91-9126693169; fax: +91-384222479.
E-mail address: tankeshwarprasadg@gmail.com