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COMMUNICATION
Superamphiphobic Polymeric Surfaces Sustaining
Ultrahigh Impact Pressures of Aqueous High- and Low-
Surface-Tension Mixtures, Tested with Laser-Induced
Forward Transfer of Drops
Kosmas Ellinas, Marianneza Chatzipetrou, Ioanna Zergioti, Angeliki Tserepi,
and Evangelos Gogolides*
K. Ellinas, Dr. A. Tserepi, Dr. E. Gogolides
Institute of Nanoscience and Nanotechnology
NCSR “Demokritos”
153 10 Aghia Paraskevi, Attiki, Greece
E-mail: e.gogolides@inn.demokritos.gr
M. Chatzipetrou, Prof. I. Zergioti
National Technical University of Athens
Physics Department
Iroon Polytehneiou 9, 15780 Zografou, Athens, Greece
DOI: 10.1002/adma.201405855
can sustain ultrahigh drop impact pressures (tens to hundreds
of atmospheres).
[12]
However, lotus-leaf surfaces remain the
only solution in applications incompatible with the use of liq-
uids used in the SLIPS surfaces.
Many techniques to probe the thermodynamic sta-
bility of artificial superamphiphobic surfaces have already
been employed,
[21]
such as: pressure experiments,
[22]
drop
impact,
[23,24]
electrowetting experiments,
[25]
or underwater
immersion,
[16]
but most of them are limited as far as the max-
imum pressure that can be induced. The laser-induced forward
transfer (LIFT) technique is commonly used for biomolecule
printing applications.
[26]
Liquid jets created by LIFT can reach
extremely high speeds exceeding 270 m s
-1
.
[27]
The impact of
such a jet on a solid surface creates a dynamic pressure as high
as 35 MPa (350 atm), enabling sticking of droplets on super-
hydrophobic surfaces and evaluation of the critical pressure
threshold for the transition from Cassie–Baxter (CB) to the
Wenzel (W) regime. Previously, LIFT has been used to make
droplets stick on random, plasma textured for few minutes
(<10 min), superhydrophobic surfaces, using very high laser
fluences (up to 1300 mJ cm
-2
).
[27]
Here, we produce hierarchical micro-nanotextured random
or (quasi-)ordered material surfaces using plasma etching as
described in the Supporting Information and in previous pub-
lications.
[28]
The method is generic and can be applied on any
polymeric material surface, poly(methyl methacrylate) (PMMA)
being the example material surface used in this work. To char-
acterize these material surfaces, we adapt the LIFT method to
probe systematically their thermodynamic stability and estimate
the pinning pressure for a wide range of mixtures with surface
tension between 36 and 66 mN m
-1
. We present evidence that
careful surface topography design (spacing, diameter, height,
and re-entrant profile of the sub-micrometer columns and for-
mation of nanoscale roughness, i.e., geometrical parameters
that can be controlled by the etching process), in combination
with a defect-free hydrophobic coating can lead to superamphi-
phobic surfaces with extreme pressure and mechanical endur-
ance exceeding 36 atm for phosphate buffer (i.e., more than
five times higher than the state-of-the-art,
[2]
and 7 atm for a low-
surface-tension buffer/propanol mixture (36 mN m
-1
) (orders
of magnitude higher than previously reported for oils
[19]
even
after ten simultaneous high velocity impacts on the same area,
expanding their spectrum of potential applications.
The development of material surfaces repelling a wide range
of liquids has attracted scientific attention for over a decade.
Lotus leaf-like and other biomimetic materials with superhy-
drophobic, and superoleophobic properties have been prepared,
and many reports about such artificial superamphiphobic
(superoleophobic and superhydrophobic) materials exist in
the literature.
[1–4]
These materials are important in many fields
of applications as described in some recent review papers.
[5,6]
Nowadays, the main focus is given in the characterization of
such surfaces
[7]
and in the optimization of their mechanical,
[8,9]
environmental,
[10]
chemical,
[11]
and thermodynamic robust-
ness.
[12]
This consistent effort has produced a wide range of
new testing methods and optimized materials with respect to
their mechanical and environmental stability as well as their
chemical resistance to organic solvents.
[11,13–18]
The “lotus-
leaf” type of surfaces allow the rolling of water and oil drops
on them, but are usually impregnated when drops impact on
them with a large pressure, or when they are submerged in liq-
uids at a high pressure (or large depth). Nevertheless, a recent
review paper
[2]
shows that examples of lotus-leaf-inspired sur-
faces, exhibiting stability against high water pressures reaching
7 atm, exist in the literature, raising hopes for improved perfor-
mance of lotus-leaf surfaces. However, resistance to the impact
of drops of liquids or mixtures with low surface tension (similar
to that of oils or alkanes) is even more difficult, and the highest
reported pressures are well below 1 atm for low-surface-tension
liquid droplets with low impact velocities.
[19]
Recent studies
suggest that implementation of nanoscale roughness is essen-
tial to achieve high thermodynamical stability.
[16,20]
An alterna-
tive solution would be to replace air with a liquid to impregnate
the micro- and nanotopography of a material surface, the so-
called slippery liquid infused porous surfaces (SLIPS), which
Adv. Mater. 2015,
DOI: 10.1002/adma.201405855
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