  Citation: Maier, P.; Ginesta, D.; Clausius, B.; Hort, N. Observations of Microstructure-Oriented Crack Growth in a Cast Mg-Al-Ba-Ca Alloy under Tension, Compression and Fatigue. Metals 2022, 12, 613. https://doi.org/10.3390/ met12040613 Academic Editors: Menachem Bamberger and Daolun Chen Received: 26 February 2022 Accepted: 31 March 2022 Published: 2 April 2022 Publisher’s Note: MDPI stays neutral with regard to jurisdictional claims in published maps and institutional affil- iations. Copyright: © 2022 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https:// creativecommons.org/licenses/by/ 4.0/). metals Article Observations of Microstructure-Oriented Crack Growth in a Cast Mg-Al-Ba-Ca Alloy under Tension, Compression and Fatigue Petra Maier 1, * , Daniel Ginesta 1 , Benjamin Clausius 1 and Norbert Hort 2,3 1 School of Mechanical Engineering, University of Applied Sciences Stralsund, 18435 Stralsund, Germany; daniel.m.roque@hochschule-stralsund.de (D.G.); benjamin.clausius@hochschule-stralsund.de (B.C.) 2 Functional Materials, Helmholtz-Zentrum Hereon, 21502 Geesthacht, Germany; norbert.hort@hereon.de 3 Institute of Product and Process Innovation, Leuphana University Lüneburg, 21335 Lüneburg, Germany * Correspondence: petra.maier@hochschule-stralsund.de Abstract: DieMag633, a cast Mg-Al-Ba-Ca alloy, was the focus of this study. Brittle interdendritic phases strongly influenced the crack initiation and propagation under quasi-static and fatigue loading. Especially under tensile loading, the material showed a low resistance to failure. Selected fatigue loading sequences were applied to investigate their influence on crack propagation. DieMag633 in this study contained shrinkage cavities and pores of significant size and irregular distribution. Even though pores played a role in initiating the crack, it was mainly influenced by the Ba- and Ca-rich phases, being and staying much harder under deformation than the Mg-matrix. Apart from the fatigue crack propagation region under fatigue loading, there was no transgranular cracking found within the dendritic α-Mg grains. Only under compression did the dendritic α-Mg grains bridge the crack from one brittle phase to another. Transgranular cracking within the compact Ba-rich phase was very pronounced, starting with many microcracks within this phase and then connecting to the macrocrack. The lamellar Ca-rich phase showed also mainly transgranular cracking, but being small lamellae, intergranular cracking was additionally found. The hardness increase under deformation depended on the loading condition; a compression load strain-hardened the material the most. μCT analysis was applied to characterize the amount and location of the shrinkage cavities and pores in the individual gauge length. Keywords: microstructure; crack propagation; brittle phases; porosity; fatigue; μ-CT analysis 1. Introduction The die-cast Mg-Al-Ba-Ca alloy, called DieMag633, was developed as a creep resistant alloy based on Mg-Al. Rare earths elements (REE) are often chosen as alloying elements when a good creep resistance is desired in Mg-Al alloys. This is based on the formation of precipitates like Al 11 RE 3 , Al 4 RE and Al 2 RE [1,2]. Alloying with Ba and Ca replaces the expensive and limited REE, strengthening precipitates where expected. Based on AXJ520 [3] and AX52/AX53 [4], where (Mg,Al) 2 Ca precipitates strengthen the alloys, and based on Mg-Zn alloys, where alloying with Ba promotes both the formation of strengthening precipitates by stimulating the precipitate nucleation and the acceleration of the kinetics of precipitation during artificial and natural ageing [5], a Mg-Al-Ba-Ca alloy was developed as a creep resistant alloy [6,7]. In this study the DieMag633 alloy, according to their alloying elements also known as ABaX633, consists mainly of primary dendrites of α-Mg and two interdendritic phases of different morphology. Increasing the amount of Al, Ca and Ba in the DieMag-series (DieMag211, DieMag422 and DieMag633—numbers stand for amount of Al, Ca and Ba in wt.%) increases strength and creep resistance based on the increasing amount of Al 2 Ca and Mg 21 Al 3 Ba 2 [7]. In the study by Dieringa et al. [6] it can be seen that the DieMag422 Metals 2022, 12, 613. https://doi.org/10.3390/met12040613 https://www.mdpi.com/journal/metals