Cite this paper: Vietnam J. Chem., 2019, 57(3), 343-346 Article
DOI: 10.1002/vjch.201900038
343 Wiley Online Library © 2019 Vietnam Academy of Science and Technology, Hanoi & Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim
Synthesis of Valsartan as drug for the treatment of hypertension
Tran Van Chien
1,2*
, Nguyen The Anh
1
, Tran Thi Phuong Thao
1,2
Le Dac Phuong
3
, Pham Thi Tham
3
, Nguyen Quang Tung
3
, Tran Van Loc
1,2
1
Institute of Chemistry, Vietnam Academy of Science and Technology, 18 Hoang Quoc Viet Road, Cau Giay,
Hanoi, Viet Nam
2
Graduate University of Science and Technology, Vietnam Academy of Science and Technology, 18 Hoang
Quoc Viet Road, Cau Giay, Hanoi, Viet Nam
3
Hanoi University of industry, No 298 Cau Dien street, Bac Tu Liem District, Hanoi, Viet Nam
Received May 15, 2019; Accepted for publication May 30, 2019
Abstract
The synthesis of valsartan (1), one of the most currently used pharmaceutical agent in antihypertensive therapy, was
described through five steps in an overall yield of 54 % starting from 4’-methyl-2-cyanobiphenyl (2). The key step
involved tetrazole ring formation catalyzed by Lewis acid. The structures of synthesized compounds were confirmed by
means of NMR and MS spectroscopíe.
Keywords. Valsartan, antihypertension, biphenyltetrazole, Lewis acid.
1. INTRODUCTION
The renin-angiotensin system (RAS) plays an
important role in the regulation of blood pressure as
well as electrolyte balance.
[1]
This system acts by
producing angiotensin I that is converted into
octapeptide angiotensin II by angiotensin-converting
enzyme (ACE). Angiotensin II is regarded as the key
regulator in stimulation of angiotensin II type 1
receptor (AT1), which mainly located in the heart,
blood vessels and kidneys, and thus triggers further
downstream effects and leads to vasoconstriction.
Currently, two major therapeutic approaches in the
treatment of hypertension target on angiotensin II
either by inhibition of angiotensin-converting
enzyme (ACE) or by blocking the action of
angiotensin II on its AT1 receptor.
[2]
Sartan drugs
such as telmisartan, candesartan, olmesartan,
irbesartan and valsartan are effectively used in the
clinic for the regulation of high blood pressure.
[3,4]
They are biphenyl-tetrazole derivatives and specific
angiotensin II antagonists, binding to the AT1
receptor subtype. Among these, valsartan has been
prescribed for the treatment of hypertension since
1996. It is commercially available in the market
under the brand name DIOVAN™ and is a generic
medication. In 2016, it was on the top 100 most
prescribed drugs in the United States of America,
with more than 8 million prescriptions. Herein, we
describe a simple synthetic procedure of valsartan in
order to develop in large pilot plant.
2. MATERIALS AND METHODS
All chemicals and solvents were purchased from
commercial suppliers and used without further
purification. Column chromatography was
performed using silica gel (60 Å, particle size 40-60
µm). NMR spectra were recorded on a Bruker
Avance 500 MHz spectrometer. Chemical shifts (δ)
are given in parts per million (ppm) and coupling
constants (J) in hertz (Hz). ESI-MS was carried out
on an Agilent 1100 mass spectrometer (Canton,
Massachusetts, USA).
Synthesis of 5-(4'-methyl-[1,1’-biphenyl-2-yl]-1H-
tetrazole (3)
A solution of 4’-methyl-2-cyanobiphenyl (2) (2.4 g,
12.44 mmol) in DMF (50 mL) was added Et3N*HCl
(3.43 g, 25 mmol) and NaN3 (2.02 g, 31 mmol). The
reaction mixture was then warmed up to 120
o
C for
54 h. The solvent was evaporated under reduced
vacuum to dryness. The residue was dissolved in
water and added aqueous solution 4 % K2CO3. The
starting material was precipitated and collected by
filtration. The filtrate was acidified with 5 % HCl.
The resulting solid was collected and dried at 65
o
C
for 4 h to obtain a white product 3 (2.8 g, 96.4 %).