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IEEE JOURNAL OF PHOTOVOLTAICS 1
Two-Dimensional Model for Perovskite Nanorod
Solar Cells: A Dark Case Study
Nouran M. Ali , Tamer A. Ali, and Nadia H. Rafat, Senior Member, IEEE
Abstract—Nanorod geometry has witnessed a massive focus in
the past few years for enhancing the solar cells performance.
It improves the cell efficiency because of the carrier transport
perpendicular to light absorption directions. Perovskite materials,
such as the methylammonium lead iodide also have attracted great
attention because of the low cost, simple manufacture process,
and good optical properties. These advantages of both nanorod
structures and perovskite materials imply that PNSC is a very
promising candidate in energy harvesting applications. This in-
creases the demand for accurate and fast models for the analysis
and for the optimization of these cells. In this article, we present an
analytical model for nanorod solar cells. The model solves the semi-
conductor equations (Poisson’s equation and continuity equations)
in two-dimensional cylindrical coordinates. It is based on using the
conformal mapping theory as an approximation for potential and
electric field estimation. It also uses separation of variables process
in solving the two-dimensional continuity equation for both radial
and axial directions. The analytical model was applied on a TiO
2
/
perovskite / spiro-MeOTAD cell to produce the dark current. The
results of this model were compared with that of a numerical finite
element model and achieved good matching.
Index Terms—Conformal mapping, continuity equations,
perovskite, photovoltaic, radial structure, Runge–Kutta method.
I. INTRODUCTION
I
N THE past few years, perovskite nanorod solar cells (PNSC)
was considered a high topic in the solar energy harvesting
research [1]. Nanorod geometry, in which the light is absorbed
in the axial direction and the carriers are collected in the radial
direction, allows an effective optical absorption, and simultane-
ous good collection of generated carriers [2]. Although silicon
is considered the dominant material in photovoltaic solar cells
with the record efficiency of 26.6% [3]–[5], perovskite solar
cells (PSCs) had a rapid increase in efficiency that makes it a
very promising choice [6]–[9]. As shown in Fig. 1, the efficiency
of PSC started from 3.8% in 2009 [6] that reaches 24.2% in 2019
[1] with a predicted efficiency limit of 31% [7].
Manuscript received July 23, 2019; revised September 4, 2019; accepted
September 6, 2019. (Corresponding author: Nouran M. Ali.)
N. M. Ali and N. H. Rafat are with the Engineering Mathematics and Physics
Department, Faculty of Engineering, Cairo University, Giza 12613, Egypt
(e-mail: eng.nouranmohamed@gmail.com; nhrafat@ieee.org).
T. A. Ali is with the Engineering Mathematics and Physics Department,
Faculty of Engineering, Cairo University 12613, Giza, Egypt, and also with
the Zewail City of Science and Technology, Giza 12578, Egypt (e-mail:
tali@zewailcity.edu.eg).
Color versions of one or more of the figures in this article are available online
at http://ieeexplore.ieee.org.
Digital Object Identifier 10.1109/JPHOTOV.2019.2940852
Fig. 1. Power conversion efficiency versus years for PSC and Si solar cells.
It is worthy to be mentioned that in 2019, silicon / perovskite
tandem cell achieved an efficiency of 27.3% [10]
The general chemical formula for perovskite compounds is
ABX
3
, where “A” and “B” are two cations of very different
sizes, and X is an anion that bonds to both [11].
Nanorods geometry enhances the performance of organic
cells [12], and inorganic cells [13], [14]. For silicon nanowire
cells, improvement in external quantum efficiency and absorp-
tion efficiency were observed experimentally [15], analytically
[16], and numerically when compared with conventional planar
p-i-n thin-film Si solar cells [17].
Analytical modeling is a very efficient method to estimate
solar cell performance. It concerns with the basic principles and
equations that governs the nanorod solar cells (NRSC). Although
perovskite cells are configured similar to the conventional solar
cells, their operations are unique and require new models for
cell characterization, and optimization [18].
Analytical models for nanorod structures started in 2005.
Kayes and Atwater [16] showed analytically that extremely
large efficiency enhancement (from 1.5% to 11%) for silicon
cells can be achieved by applying the radial geometry. Then,
in 2012, another analytical model was developed by Petrosyan
et al. [19], where they calculated the potential distribution, and
derived expressions to compute the depletion region width and
capacitance. In 2014, other studies presented an analytical model
based on Green’s function theory to calculate the current density,
open circuit voltage, fill factor, and conversion efficiency [20],
[21]. The use of Green’s function reduced the need for uniform
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