FEMS MicrobiologyLetters 42 (1987) 27-31 27
Published by Elsevier
FEM 02764
The Pasteur effect in yeasts: mass spectrometric monitoring of
oxygen uptake, and carbon dioxide
and ethanol production
D. Lloyd and C.J. James
Department of Microbiology, University College, Newport Road, Cardiff U.I(
Received and accepted 9 January 1987
Key words: Saccharomyces eerevisiae," Saccharomyces uvarum; Pasteur effect; Glycolysis; Fermentation;
(Mass spectrometry)
1. SUMMARY 2. INTRODUCTION
Simultaneous and continuous monitoring of
dissolved 02, CO 2 and ethanol in suspensions of
Saccharomyces uvarum and Saccharomyces cere-
visiae, by means of a quadrupole mass spectrome-
ter fitted with a silicone rubber membrane inlet,
enabled a study of 0 2 inhibition of glycolysis
(Pasteur effect). Calculation of Pasteur quotients
(ratios of anaerobic to aerobic glycolytic rates)
give similar values when corrected both for re-
spiratory CO 2 production and ethanol oxidation
under aerobic conditions. For S. cerevisiae the
apparent K m for 0 2 of the respiration of catabo-
lite derepressed cells was 1 /~M and the apparent
K i values for O 2 as an inhibitor of glycolysis were
12.7 and 7/~M, respectively, when measurements
were made on CO 2 evolution and ethanol produc-
tion.
Correspondence to: D. Lloyd, Dept. of Microbiology, Univer-
sity College, Newport Rd., Cardiff, CF2 1TA, Wales, U.K.
The inhibition of glycolysis by 0 2 has been
extensively studied in a wide variety of organisms
and tissues [1], but the exact nature of the control
mechanisms involved is still debated [2,3]. This
Pasteur effect, originally discovered in yeast [4] is
easily investigated in that organism which shows
rapid and pronounced responses to changes in
sugar or 0 2 concentrations [5,6]. S. cerevisiae has
the added advantage that many mutant strains
defective in different enzymes of glycolysis have
been isolated [7]. Despite these advances, and the
identification of several key control points, e.g.,
hexose transport [8], phosphofructokinase [9,10],
pyruvate/kinase [11], and NAD+-dependent iso-
citrate dehydrogenase [12], many aspects of the
Pasteur effect remain unexplained. We report here
a technique that greatly facilitates research on the
Pasteur effect, a continuous and simultaneous mass
spectrometric monitoring of 0 2, CO 2 and ethanol
dissolved in yeast suspensions. When performed
under carefully controlled conditions of gas ex-
change [13], rate measurements on all 3 compo-
nents may be determined under aerobic or
anaerobic conditions, or at very low 0 2 concentra-
0378-1097/87/$03.50 © 1987 Federation of European Microbiological Societies