FULL PAPER
Novel thin film nanocomposite membranes incorporated
with polyoxovanadate nanocluster for high water flux and
antibacterial properties
Mojtaba Amini
1
| Zahra Shekari
1
| Ali Akbari
2,3
| Hadi Naslhajian
1
|
Ayda Sheykhi
1
| Esmaeil Karimi
4
| Sanjeev Gautam
5
| Keun Hwa Chae
6
1
Department of Chemistry, Faculty of
Science, University of Maragheh,
Maragheh, Iran
2
Cellular and Molecular Research Center,
Research Institute for Cellular and
Molecular Medicine, Urmia University of
Medical Sciences, Urmia, Iran
3
Solid Tumor Research Center, Cellular
and Molecular Medicine Institute, Urmia
University of Medical Sciences, Urmia,
Iran
4
Department of Soil Science, Faculty of
Agriculture, University of Maragheh,
Maragheh, Iran
5
Dr. S.S. Bhatnagar University Institute of
Chemical Engineering & Technology,
Panjab University, Chandigarh, 160-014,
India
6
Advanced Analysis Center, Korea
Institute of Science and Technology,
Seoul, 136-791, South Korea
Correspondence
Mojtaba Amini, Department of
Chemistry, Faculty of Science, University
of Maragheh, Maragheh, Iran.
Email: mamini@maragheh.ac.ir
Using interfacial polymerization (IP) of m-phenylenediamine aqueous solution
containing polyoxovanadate nanoclusters (POV) and trimesoyl chloride (TMC)
in organic solution, we fabricated a novel polyamide (PA)- polyoxovanadate
nanocluster (POV) nanocomposite membranes (PA-POV TFN). The chemical
structures and morphologies of the synthesized membranes were characterized
by Fourier transform infrared (FTIR) spectroscopy, atomic force microscope
(AFM), scanning electron microscopy (SEM) and water contact angle measure-
ments. Experimental results showed that the performances of PA-POV TFN
membranes are remarkably dependent on POV incorporation in the mem-
branes, which could be controlled by using different amounts of POV particles.
Moreover, the PA-POV TFN membranes illustrated outstanding antibacterial
properties against Gram-negative E. coli. On the other hand, the incorporation
of various amounts of POV in the membranes improved the membrane separa-
tion performances (water flux and salt rejection) as well as the antibacterial
activity in FO process as compared to the original thin-film composite (TFC)
polyamide membrane.
KEYWORDS
Polyoxovanadate, antibacterial property, desalination, interfacial polymerization, membrane
1 | INTRODUCTION
Presently, more than 650 million global populations suf-
fer from inadequate safe and clean drinking water.
[1]
Based on the United Nations report,
[2]
it is predicted that
half of the worldwide people will be staying in the areas
of high freshwater scarcity by 2030, resulting in a great
threat to the sustainable development of human society.
Thus, membrane technology could be considered as one
of the most powerful tools for water desalination due to
its high stability, efficiency, low cost, easy operation and
low energy consuming.
[3]
Various types of separation
membrane such as reverse osmosis membrane (RO),
nanofiltration membrane, ultrafiltration membrane,
microfiltration membrane and forward osmosis mem-
brane (FO) have been developed,
[4]
which among these,
forward osmosis (FO) as a novel membrane technology
(using natural osmotic pressure as a driving force) has
many advantages including, low cost,
[5]
easy cleaning,
[6]
low fouling tendency
[7]
and so on. It is noteworthy that
high fouling tendency, low hydrophilicity and poor per-
formance of FO membranes limited their industrial
Received: 3 September 2019 Revised: 8 December 2019 Accepted: 11 December 2019
DOI: 10.1002/aoc.5494
Appl Organometal Chem. 2020;e5494. wileyonlinelibrary.com/journal/aoc © 2020 John Wiley & Sons, Ltd. 1 of 8
https://doi.org/10.1002/aoc.5494