Int. J. Pharm. Investigation, 2022; 12(3) : 328-333
328 International Journal of Pharmaceutical Investigation, Vol 12, Issue 3, Jul-Sep, 2022
Original Article
INTRODUCTION
Tese studies examined mutual protective relationships among rabbit
muscle aldolase, enolase, phosphofructokinase-1 (PFK-1) and LDH
from inhibitions by ascorbate (AA). It was proposed earlier
1-2
that
specifc inhibitions of PFK-1 and LDH by AA faciltated glycogen storage
in resting muscle by inhibiting glycolysis. A ten step metabolic pathway
i.e. Glycolysis is catablozed by the pyruvate that leads to the production
of energy i.e. adenosine tri phosphate (ATP ) and nicotine adenine
dinucleotide (NADP). Te breakdown of aaldol cleavage is the fourth
step of glycolysis in which 6 free carbon of fructise 1,6 bisphosphate in
to 2. Te two are glyceraldehyde 3- phosphatte and dihydoxyacetone
phosphate.
3
Aldolase were found in various types of bacteria and
eukaryotes. It has important role not only in glycolysis but also in
gluconeogenesis and metabolism of fructise.
4-5
Earlier studies
4
also showed that activity losses due to inhibition by
AA and due to dilution,
5-6
were prevented by the presence of rabbit
muscle aldolase. Rexaminations of enolase and other glycolytic enzymes
inhibitons by AA were undertaken to determine whether or not
inhibitions of enolase by AA were also prevented by aldolase.
A report by others
7-8
that a AA-fatty acid derivative inhibited cancer
growth efects of other AA-fatty acid derivatives on enolase activity.
Mutual protection of PFK-1, aldolase, enolase and LDH from inhibitions
were investigated. Comparitive studies of enolase and aldolase efects on
PFK-1 activity loses by dilutions, by AA inhibitions, and by AA fatty acid
inhibitions were made.
MATERIALS AND METHODS
Materials
Te L-ascorbate (AA), L-ascorbyl dibutyrate (AADB), L-ascorbyl
dipalmitate (AADP), L-ascorbyl palmitate (AAP), and L- ascorbyl
stearate (AS) are shown in Figure 1 and were obtained from TCI and Alfa
Aesar. Enzymes and materials given below were from Sigma (catalog
numbers) unless stated otherwise.
Methods
Unless otherwise stated, all enzymes come from rabbit and all
experimental temperatures were 25°C, pH 8.0. Compared to the main
enzyme activity, it was determined that enzyme enolase (E0379)
contained activities ≥ 0.05% by LDH or by PFK-1; LDH contained ≥
0.01% enolase activity; and aldolase (A8811) contained ≥ 0.05% PFK-1.
AA-fatty acid derivatives were dissolved in ethanol or dimethyl sulfoxide
(DMSO, D8418). It can be shown that neither 15% ethanol nor 15%
DMSO inhibited any enzymes used in these studies, more than the upper
limit of the solvents used. Minimum six experiemnts were performed.
Less than ± 10% standard deviation from the mean (SEM) than Data
were acceptable. ± 10% error bars represent the SEM.
Rabbit Muscle PFK-1 Preparation
Purifed rabbit muscle PFK-1 in these experiments was presented
previously
5
according to the method of Kemp
9
and stored as a 60%
saturated ammonium precipitate until ready for use. A single band in
SDS PAGE was used for PFK-1 samples in all muscle of rabbit as shown
Inhibition by Ascorbate among Phosphofructokinase-1,
Aldolase, Enolase, and Lactate Dehydrogenase in Rabbit Muscle
Anita Ricablanca
1
, Ami Abbott
1
, Fatimata Sonago
1
, Montserrat Garcia
1
, Rachel Primacio
1
, Eric Patten
1
, Mudassar Iqbal Arain
2
,
Eduardo Fricovsky
2,
*
1
Department of Medical Education, School of Medicine University of California, San Diego, La Jolla, CA 92093, USA.
2
Skaggs School of Pharmacy and Pharmaceutical Sciences, University of California San Diego, San Diego, La Jolla, CA, USA.
ABSTRACT
Background: These studies examined mutual protective relationships
among rabbit muscle aldolase, enolase, phosphofructokinase-1 (PFK-1)
and LDH from inhibitions by ascorbate (AA). It was proposed earlier that
specifc inhibitions of PFK-1 and LDH by AA faciltated glycogen storage
in resting muscle by inhibiting glycolysis. Materials and Methods: The
L-ascorbate (AA), L-ascorbyl dibutyrate (AADB), L-ascorbyl dipalmitate
(AADP), L-ascorbyl palmitate (AAP), and L- ascorbyl stearate (AS) are shown
in Figure 1 and were obtained from TCI and Alfa Aesar. Unless otherwise
stated, all enzymes come from rabbit and all experimental temperatures
were 25°C, pH 8.0. Results: Rabbit muscle enolase was examined for
its protective effect on other rabbit muscle glycolytic enzymes against
inhibitions by ascorbate (AA) and some AA-faty acid derivatives. The
IC
50
values of enolase by ascorbate (AA) and IC
50
values of AA-fatty acid
derivatives were compared to estimate inhibition potency. For example,
ascorbyl dipalmitate (AADP) was 156 times more inhibitory to enolase
than AA. It was previously shown that rabbit muscle aldolase prevented
LDH activity loses due to AA inhibition and prevented PFK-1 activity losses
due both to dilution and AA inhibition; enolase was found to have the
same effects as aldolase. Additionally, PFK-1 prevented enolase and LDH
inhibitions by AA. LDH did not prevent enolase or PFK-1 from inhibition by
AA. LDH did stimulate enolase activity but not PFK-1 activity. Conclusion:
The results suggest that interactions among glycolytic enzyme serve to
mutually protect one another from activity losses. The inhibition properties
of the AA-fatty acid derivatives are discussed in relation to their possible
roles in cancer and diabetes.
Keywords: Phosphofructokinase-1, Aldolase, Enolase, Ascorbate, Rabbit.
Correspondence
Dr. Eduardo Fricovsky
Professor of Clinical, University of California, San Diego, La Jolla,
CA 92093-0690, U.S.A.
Email id: esfricovsky@health.ucsd.edu
DOI: 10.5530/ijpi.2022.3.55
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