Presented at the International Congress on Membranes and Membrane Processes (ICOM), Seoul, Korea,
21–26 August 2005.
0011-9164/06/$– See front matter © 2006 Elsevier B.V. All rights reserved
Desalination 193 (2006) 160–165
Bergamot essential oil extraction by pervaporation
A. Figoli
a*
, L. Donato
a
, R. Carnevale
a
, R. Tundis
b
, G.A. Statti
b
, F. Menichini
b
,
E. Drioli
a
a
Institute of Membrane Technology, Via P. Bucci 17/c, 87036 Rende (Cs), Italy
Tel. +39 (0984) 492027; Fax: +39 (0984) 402103; email: a.figoli@itm.cnr.it
b
Department of Pharmaceutical Sciences, University of Calabria, 87036 Rende (CS), Italy
Received 24 March 2005; accepted 27 June 2005
Abstract
Bergamot peel oil is the most valuable essential oil due to its unique fragrance and freshness. The essence finds
application in the cosmetic, pharmaceutical and food industries. However, strong limitations have been imposed on
its use since bergamot oil contains several coumarins and psoralens which may be photoactive. Qualitative and
quantitative analyses with GC–MS were carried out to evaluate the aroma flavour bouquet of the bergamot essential
oil obtained by pervaporation (PV). In all PV experiments, made at different ethanol feed concentration and
temperature, the bergapten was not detected in the permeate while the aroma components, present in the feed, permeate
through the commercial Pervap 1070 membrane. Bergapten is a photoactive component of bergamot essential oil
which, in combination with UV radiation, promotes melanogenesis and causes thickening of the stratum corneum.
Therefore, PV is a valid alternative for the high quality of essential oil produced without bergapten to the traditional
techniques employed in which the bergapten can be removed after an extra-chemical treatment.
Keywords: Bergamot; Pervaporation; Essential oil; Aroma recovery; Hydrophobic membrane; Extraction technique
1. Introduction
The extraction of aroma compounds from
natural matrixes by pervaporation (PV) represents
a valid alternative to techniques commonly used
such as steam distillation and liquid solvent
*Corresponding author.
extraction. Due to its high selectivity, PV allows
the recovery at low temperature the aroma com-
pounds preserving the molecule integrity, its high
selectivity and respecting the environment (no
solvent use, low energy consumption) [1–3].
Citrus peel oils are widely used in the perfume
and cosmetic industries. Among them, bergamot