Mutation Research, 207 (1988) 135-139 135
Elsevier
MTR 04575
Effect of copper coordination complexes
on sister-chromatid exchanges in plant cells
M.J. Hazen, A. Juarranz, J.C. Stockert, A. Gonzalez and D. Beltrfin-Porter
Departamento de Biologla, Facultad de Ciencias, Universidad A utbnoma de Madrid, Madrid, and Departamento de Qulmica Inorgtinica,
Facultad de Quimica, Universidad de Valencia, Valencia (Spain)
(Received 15 July 1987)
(Revision received 22 September 1987)
(Accepted 14 October 1987)
Keywords: Copper coordination complexes; Plant cells, SCE; Sister-chromatid exchanges, plants.
Summaff
The effectiveness of several copper coordination complexes in the induction of sister-chromatid
exchanges (SCE) in meristematic cells of Allium cepa roots was studied. A significant increase in the
frequencies of SCE was observed when cells were exposed to different concentrations of copper complexes
for 3 h. This effect, which is concentration dependent, seems to be related to the possibility of intercalative
binding modes between the planar copper complexes and DNA.
The phenomenon of sister-chromatid exchanges
(SCE) has constituted the subject of many reports
during the last years (for review see Kato, 1977;
Wolff, 1977; Latt, 1979; Latt et al., 1981). Al-
though SCE are commonly used as a short-term
mutagen-carcinogen test, their biological rele-
vance and mechanism of formation are still not
well understood (see Painter, 1980). Various chem-
ical and physical agents have been found to cause
damage to chromosomal DNA, which can be cyto-
logically detected by an increase in the frequency
of SCE (Latt et al., 1979, 1981). Likewise, com-
pounds which bind to DNA by intercalation are
potent SCE inducers (Latt and Loveday, 1978;
Raj and Heddle, 1980; Cortes and Hazen, 1984;
Armas-Portela et al., 1985; Villanueva et al., 1986).
A complex between the chelating agent 1,10-
Correspondence: Prof. Dr. Juan C. Stockert, Departamento de
Biologla, Facultad de Ciencias, C-XV, Universidad Aut6noma
de Madrid, Cantoblanco, Madrid-28049 (Spain).
phenanthroline (OP) and copper(II) is able to
induce in vitro the breakage of DNA strands in
the presence of a reducing agent and 02 or H202
(Que et al., 1980; Graham et al., 1980; Marshall et
al., 1981; Pope et al., 1982). This process is in-
hibited by intercalating dyes and catalase and it
does not occur when highly stabilized Cu(I) or
Cu(II) complexes are used (Que et al., 1980;
Marshall et al., 1981). Although the mechanism of
DNA breakage has not yet been fully determined,
it is assumed that the Cu(I)-OP complex inter-
calates into DNA (Marshall et al., 1981; Uesugi et
al., 1982), and that subsequent oxidation by H202
originates the scission of DNA due to the forma-
tion of a highly reactive hydroxyl radical at the
binding site (Goldstein and Czapski, 1986). Cu-OP
is capable of recognizing and cleaving DNA from
nucleosomes and chromatin (Elgin et al., 1983),
showing interesting applications as a quasi-en-
zymatic agent (Drew and Travers, 1984; Chen and
Sigman, 1986).
0165-7992/88/$03.50 © 1988 Elsevier Science Publishers B.V. (Biomedical Division)