* Corresponding author: Dehno Khalaji, Aliakbar E-mail: alidkhalaji@yahoo.com © 2021 by SPC (Sami Publishing Company) Advanced Journal of Chemistry-Section A Journal homepage: www.ajchem-a.com Original Research Article Effective Removal of Methyl Green from Aqueous Solution Using Epichlorohydrine Cross-Linked Chitosan Zahra Bashandeh, Aliakbar Dehno Khalaji* Department of Chemistry, Faculty of Science, Golestan University, Gorgan, Iran A R T I C L E I N F O A B S T R A C T Article history Submitted: 09 May 2021 Revised: 27 June 2021 Accepted: 08 July 2021 Available online: 11 July 2021 Manuscript ID: AJCA-2105-1259 DOI: 10.22034/AJCA.2021.285520.1259 Epichlorohydrin cross-linked chitosan (EP-Cs) was prepared was characterized using Fourier transform infrared spectroscopy (FT-IR), X-ray powder diffraction (XRD), thermal gravimetry (TG-DTA) and differential calorimetric analysis (DSC), and used as adsorbent for methyl green (MG) removal. Epy-Chit was soaked in methyl green solution with concentration of 40 mg/L using a batch adsorption system, to measure the adsorption capacity of the EP-Cs and the percentage of MG removed from the aqueous solution. The optimum MG adsorption on EP-Cs occurred at pH 7.8, agitation time of 60 minute and adsorbent dosage of 0.02 g were observed. Adsorption results show that the EP-Cs exhibited the excellent performance for the MG removal from aqueous solution. This study suggests that EP-Cs could be explored as an adsorbent for removing other organic pollutants. K E Y W O R D S Epichlorohydrin Cross-linked Chitosan Adsorbent Methyl green G R A P H I C A L A B S T R A C T O O O NH 2 O H * * n O O O N H 2 OH * * n O H Cl O O O H O N H 2 OH * * n Advanced Journal of Chemistry-Section A, 2021, 4(4), 270-277