SOLUBILITY OF ALUMIMA IN HYDROXIDE - SALT MELTS
Oleg G. Zarubitskii and Igor N. Skryptun
V.I.Vemadskii Institute of General and Inorganic Chemistry
National Academy of Sciences of the Ukraine,
32-34 Palladina Ave, Kiev-142, Ukraine, 03680
ABSTRACT
Used method of isothermal saturation solubility of aluminium oxide
in alkali and alkaline-salt melts has been investigated at temperature range
673 - 873 K. It was determined that solubility of AI2O3 in the order of
melts LiOH - KOH - NaOH - (0.5KOH - 0.5NaOH) are increased. The
effect of temperature on the AI2O3 solubility in alkali melts are described
of the equation of straight line In C = A - B/T, where C is concentration of
the AI2O3 in the melts, mole fract., A and B are constants. It was indicated
that when alumina is dissolved in alkali melts, the solutes are alkaline
meta-aluminates. The salt additions of sodium chlorine, potassium
chloride, sodium carbonate and sodium, nitrate to sodium hydroxide melt
are decreased the solubility of alumina. It was calculated the
thermodynamic parameters of process solubility of aluminium oxide in
alkali hydroxide melts.
INTRODUCTION
In the past melts of alkali hydroxides and their mixture with salts were widely used
in industry for removing alumina-based ceramics from metal surfaces (1). Besides the
regularity of process solubility these systems are of interest for ionic melts chemistry.
Only a few papers addressing the interaction of aluminium oxide with alkali metal
hydroxides have been published (2 - 6). Goret and Tremillon (2) measured the solubility
of alumina in a molten eutectic mixture of sodium and potassium hydroxides at 500 K.
They proposed that alumina dissolved with chemical interaction and production of
sodium meta-alumunates. In (3 - 6) the kinetics of interaction of aluminium oxide with
alkali hydroxides by differential thertmogravimetric method are reported. It was shown
that in this process the only products are alkaline meta-aluminates. However, in the
literature there are no data on the solubility of alumina in alkali and alkaline-salt melts.
This investigation was undertaken to examine the process in this systems.
Proceedings of The Electrochemical Society, PV 1999-41, 368-375 (1999)
DOI: 10.1149/199941.0368PV © The Electrochemical Society
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