Frontiers in Science 2012, 2(6): 235-242
DOI: 10.5923/j.fs.20120206.17
Comparative Study of Indion-AGR and Duolite A-638
Anion Exchange Resins by Application of
131
I and
82
Br as
a Tracer Isotopes
Pravin U. Singare
Department of Chemistry, Bhavan’s College, Munshi Nagar, Andheri (West), Mumbai, 400 058, India
Abstract The present study deals with modeling of ion-isotopic exchange reaction kinetics by application of
radioactive tracer isotopes 82Br and 131I. The bromide and iodide ion-isotopic exchange reactions was carried out by using
weak base anion exchange resins Indion-AGR and Duolite A-638. It was observed that for both the resins, reaction rate
decreases with rise in temperature and increases with increase in ionic concentration. The study was extended further for
characterization of these resins based on their performance under different operational parameters. It was observed that the
percentage/amount of ions exchanged and distribution coefficient values calculated for Duolite A-638 was higher than
Indion-AGR resins under identical operational parameters, indicating superior performance of Duolite A-638 over
Indion-AGR resins.
Keywords Indion-AGR, Duolite A-638, Tracer Applications, Reaction Kinetics, Ion-Isotopic Exchange Reactions,
131
I,
82
Br, Distribution Coefficient, Reaction Rate
1. Introduction
Radioisotopes find applications in several fields of which
industrial applications constitute a major portion with
respect to the quantum of activity used and the economic
benefits accrued. Industrial applications of radioisotopes can
be mainly categorized into two. The first one being the use of
radiation from sealed sources of radioisotopes or from
electron beam accelerators for industrial processing,
non-destructive testing. The second major group of
applications is the use of radiotracers in inventory control,
study of process parameters, trouble shooting in industrial
systems, flow measurements, leakage studies etc. The
economic benefits that may be derived from the use of the
radioisotope technology are great, a fact that is recognized by
the governments of developing countries. Though
radioisotopes have been applied to the solution of problems
in industry for over 50 years, research and development of
the technology continues unabated. There are two main
reasons for the continuing interest. Firstly, it is industry
driven. Because of their unique properties, radioactive
isotopes can be used to obtain information about plants and
processes that cannot be obtained in any other way. Often,
the information is obtained with the plant on-stream and
* Corresponding author:
pravinsingare@gmail.com (Pravin U. Singare)
Published online at http://journal.sapub.org/fs
Copyright © 2012 Scientific & Academic Publishing. All Rights Reserved
without disrupting the process in any way. This can lead to
substantial economic benefits, from shutdown avoidance to
process optimization. Secondly, the methodology is derived
from many fields of science and technology including
radioisotope production, radiation detection, data acquisition,
treatment and analysis, and mathematical modeling.
The fundamental principle in radiochemical investigations
is that the chemical properties of a radioisotope of an element
are almost the same as those of the other stable/radioactive
isotopes of the element. When radioisotope is present in a
chemical form identical to that of the bulk of the element in a
chemical process, then any reaction the element undergoes
can be directly traced by monitoring the radioisotope.
Radiochemical work involves two main steps first is the
sampling of chemical species to be studied and second is
quantitative determination of the radiation emitted by the
radioisotope in the sample[1]. In radiotracer study, a short
lived radioisotope in a physico-chemical form similar to that
of the process material is used to trace the material under
study. The radioisotopes in suitable physical and chemical
forms are introduced in systems under study. By monitoring
the radioactivity both continuously or after sampling
(depending on the nature of study), the movement,
adsorption, retention etc. of the tracer and in turn, of the bulk
matter under investigation, can be followed. The tracer
concentration recorded at various locations also helps to
draw information about the dynamic behavior of the system
under study. The radioisotopes preferred for such studies are
gamma emitters having half-life compatible with the