Vol.:(0123456789) 1 3
Bioprocess and Biosystems Engineering
https://doi.org/10.1007/s00449-019-02211-9
RESEARCH PAPER
Antioxidant compounds extracted from Diaporthe schini using
supercritical CO
2
plus cosolvent
Barbara Vargas da Rosa
1
· Kátia Regina Kuhn
1
· Gustavo Andrade Ugalde
2
· Giovani Leone Zabot
3
·
Raquel Cristine Kuhn
1
Received: 16 April 2019 / Revised: 6 September 2019 / Accepted: 8 September 2019
© Springer-Verlag GmbH Germany, part of Springer Nature 2019
Abstract
Endophytic fungi have been highlight in the production of secondary metabolites with diferent bioactive properties, such as
in the production of the antioxidant compounds. Therefore, the objective of this work was the extraction of the antioxidant
compounds from the biomass of Diaporthe schini using supercritical carbon dioxide (CO
2
) without and with ethanol as
cosolvent. The biomass was produced by submerged fermentation and the parameters evaluated in the extraction process
were: pressure (150–250 bar), temperature (40–60 ºC) and cosolvent [biomass: cosolvent ratio, 1:0, 1:0.75 and 1:1.5 (w/v)].
Extraction yield, antioxidant activity and chemical composition of the extracts were determined. The highest extraction
yield (3.24 wt.%) and the best antioxidant activity against the 2,2-diphenyl-1-picrylhydrazyl (DPPH) radical (96.62%)
were obtained at 40 ºC, 250 bar and biomass:cosolvent ratio of 1:1.5 (w/v). The chemical compounds 1,4-diaza-2,5-dioxo-
3-isobutyl bicyclo[4.3.0]nonane and benzeneethanol identifed in GC/MS could be responsible for the antioxidant activity
found in this study.
Graphic abstract
0 5 10 15 20 25 30 35
0.0
0.4
0.8
1.2
1.6
2.0
2.4
2.8
3.2
0.00
0.02
0.04
0.06
0.08
0.10
0.12
0.14
0.16
0 5 10 15 20 25 30 35 40 45
S/F (g solvent/g feed)
Yield (wt.%)
Extract (g)
Time (min)
With co-solvent Without co-solvent
Diaporthe schini (fungus)
Extract
Submerged fermentation
Lyophilized
biomass
Supercritical
extraction
CO
2
CO
2
+ ethanol
Antioxidant
compounds
Keywords Submerged fermentation · Diaporthe schini · Supercritical CO
2
extraction · Cosolvent · Antioxidant activity
* Raquel Cristine Kuhn
raquel.kuhn@ufsm.br
Extended author information available on the last page of the article